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Record W4414293285 · doi:10.52825/solarpaces.v3i.2449

Modeling of an High-Concentration Solar Reactor for Dry Methane Reforming

2025· article· en· W4414293285 on OpenAlexafffundabout
Jean-François Dufault, Emeric Désilets, Nicolas Brissette, Nadi Braidy, Luc G. Fréchette, Mathieu Picard

Bibliographic record

VenueSolarPACES Conference Proceedings · 2025
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsUniversité de Sherbrooke
FundersFonds de recherche du Québec – Nature et technologiesHORIZON EUROPE Framework ProgrammeEuropean CommissionNatural Sciences and Engineering Research Council of CanadaMitacsEuropean Climate, Infrastructure and Environment Executive Agency
KeywordsMethaneSteam reformingSolar energyHeat fluxConcentrated solar powerPlug flow reactor modelWork (physics)Flux (metallurgy)

Abstract

fetched live from OpenAlex

Direct solar-powered reforming of methane has the potential to lower the CO2 footprint of reforming and to harvest solar energy with high-efficiency [1]. Combined with bio-sourced feedstock and recycled CO2 to perform dry methane reforming (DMR), this approach can highly decrease methane reforming environmental impact [2]. Using high solar concentration solar towers or parabolic dishes to provide the highly endothermal reaction heat required for DMR, it is possible to reach the temperatures of conventional reformers, ranging from 800°C up to 900°C. At this temperature, radiation losses are such that high solar concentrations approaching 1000x are required to reach high thermal efficiency, making heat flux management highly challenging. Previous work from Université de Sherbrooke experimentally shown the potential for such reactors to operate under high heat flux [3],[4]. The current work presents the modeling approach used to design these reactors and increase the heat flux within the absorption surface, while maintaining reasonable temperature drop within the reactor. Dimensional analysis if first assess that no diffusion limitation occurs within the reactor and the system can be simulated as a plug flow reactor with porous catalyst. Using DMR and RWGS kinetics from literature with 2D modeling in COMSOL Multiphysics, temperature and reaction rates along the reactor are evaluated showing consistency with experimental values. Parametrical analysis shows that optimal catalyst channels width appears to be equal or under 0.5 mm. Finally, it is demonstrated that optimal conversion occurs when around 1/3 of the catalytic bed is covered with metallic conductive fins. Over this value, increased conductivity gains are overpassed by the lowering of catalyst volume within the conduction chamber.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.404
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.002
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.269
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes3
Has abstractyes

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