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Record W4414300680 · doi:10.1016/j.ccst.2025.100516

An open-source dynamic model for direct air capture of carbon dioxide using solid sorbents

2025· article· en· W4414300680 on OpenAlexafffund
Shakouri Milad Kalfati, Ahmed Abdulla

Bibliographic record

VenueCarbon Capture Science & Technology · 2025
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsCarleton University
FundersGovernment of CanadaCarleton University
KeywordsSorbentCarbon dioxide removalProcess (computing)Carbon dioxideGreenhouse gasClimate change mitigationControl reconfigurationEnergy (signal processing)

Abstract

fetched live from OpenAlex

• We present a dynamic, open-source model for solid-sorbent direct air capture (DAC) • It integrates hourly, location-specific weather to predict realistic performance • Results reveal strong seasonal variation in capture performance • Energy intensity during hot periods is five times higher than during cold periods. • The model can support researchers in evaluating DAC performance in the real-world. Averting the worst consequences of climate change requires decarbonizing the global energy system and deploying carbon dioxide removal technologies, including the direct air capture of CO 2 . To estimate the cost and performance of the latter technologies, climate and energy system analysts need numerical process models that are validated with experimental data. Existing process models often limit reconfiguration that accommodates different design choices or restrict modelling to steady-state conditions. However, ambient environmental conditions like temperature, humidity, pressure, and inlet CO 2 concentration vary, affecting capture. This study develops an open-source process model for direct air capture using solid sorbents. Starting from first principles, this model allows users to select facility sizes, sorbents, other design parameters, and locations to simulate the capture performance of a solid sorbent direct air capture plant. More importantly, users can incorporate climate data to determine site-specific performance. Here, model validation is presented for two cold-climate sorbents that are being proposed for nations in northern latitudes. Results for climatically different cities are presented, highlighting the importance of sorbent choice and ambient environmental conditions on the overall capture performance and energy requirement of a direct air capture facility. The model can be employed by engineers, investors, and energy system analysts to undertake design optimization research, siting analyses, and improved studies that integrate high-fidelity process models into energy system optimization.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.483
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0030.005
Science and technology studies0.0000.002
Scholarly communication0.0000.000
Open science0.0040.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.277
Teacher spread0.266 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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