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Record W4414329552 · doi:10.37190/ppmp/210992

Adsorption behavior of fatty acids during high-density conditioning for spodumene flotation

2025· article· en· W4414329552 on OpenAlex
Brian Kawenski Cook, Luke Woolcock, Baian Almusned, Charlotte E. Gibson

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenuePhysicochemical Problems of Mineral Processing · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMinerals Flotation and Separation Techniques
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsSpodumeneAdsorptionChemisorptionPhysisorptionFatty acidLithium (medication)Polyunsaturated fatty acidFroth flotation

Abstract

fetched live from OpenAlex

The growing demand for electric vehicles and lithium-ion batteries is driving the development of new lithium projects. Spodumene, the primary lithium bearing mineral, is found in pegmatite deposits and is often recovered by froth flotation with fatty acid collectors. These collectors are known for poor selectivity, often recovering other silicate gangue minerals due to their similar surface properties when conditioning is poorly executed. High-density conditioning is a favored approach to achieve desired spodumene flotation performance with tall oil fatty acids, but the mechanisms at play during this stage are largely unknown. This study combined batch flotation with real ore samples and Time of Flight-Secondary Ion Mass Spectroscopy (ToF-SIMS) and X-ray Photoelectron Spectroscopy (XPS) analysis with single minerals, to understand the fatty acid adsorption behavior during conditioning in relation to spodumene flotation performance. The ToF-SIMS results revealed a high amount of physisorbed molecular fatty acid is needed for high spodumene recovery, but physisorption decreased as conditioning progressed, reducing lithium recovery and improving selectivity – an observation validated with two different spodumene ores. This study provides strong evidence that physical adsorption of molecular fatty acid alongside chemisorption of the fatty acid anion, either independently or as an acid-anion complex, are required on spodumene at an ideal ratio for desirable flotation performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.022
Threshold uncertainty score0.537

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.270
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it