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Record W4414372276 · doi:10.1021/acsestengg.5c00240

Microbial Response Following a Carboxymethyl Cellulose-Stabilized Sulfidated Nano Zero-Valent Iron Injection: A Long-Term Field Study

2025· article· en· W4414372276 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS ES&T Engineering · 2025
Typearticle
Languageen
FieldEngineering
TopicEnvironmental remediation with nanomaterials
Canadian institutionsCanadian Nuclear LaboratoriesWestern UniversityUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsAustralian Research CouncilDow Chemical Company
KeywordsField (mathematics)Nano-Carboxymethyl celluloseCobalt

Abstract

fetched live from OpenAlex

Sulfidated nano zero-valent iron (S-nZVI), recognized for its high remediation efficiency, was evaluated in a field trial to assess its impact on microbial communities in subsurface environments contaminated with chlorinated volatile organic compounds (cVOCs). Over a 1.5 year monitoring period, groundwater samples were collected to track microbial responses following the injection of carboxymethyl cellulose (CMC)-stabilized and dithionite-sulfidated nZVI (CMC-S-nZVI). The study observed pronounced and prolonged biostimulatory effects at locations receiving notable amounts of CMC-S-nZVI, as evidenced by increased DNA and bacterial concentrations. 16S rRNA gene sequencing revealed the selective enrichment of organohalide-respiring bacteria (OHRB), including Dehalococcoidaceae, which played a crucial role in cVOCs biotic dechlorination. Numerical ecological analyses indicated a sustained shift in microbial community structures post injection. Additionally, Fe 3+ /sulfur-reducing OHRB, including some strains of Geobacter, Sulfurospirillum, and Desulfitobacterium, emerged as major components of the total bacterial population. These microorganisms likely utilized both injected and native sulfur and iron species to form iron sulfides, potentially contributing to abiotic dechlorination. This microbially mediated process may explain the complete dechlorination of cVOCs with minimal vinyl chloride accumulation. This study demonstrates the long-term adaptation of microorganisms to the injected CMC-S-nZVI and its effectiveness in removing cVOCs through a combination of abiotic and biotic processes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.043
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.219
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it