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Influence of Added Surfactants on the Rheology and Surface Activity of Polymer Solutions

2025· article· en· W4414427448 on OpenAlex

Why this work is in the frame

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affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueChemEngineering · 2025
Typearticle
Languageen
FieldChemical Engineering
TopicRheology and Fluid Dynamics Studies
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPulmonary surfactantCationic polymerizationRheologyPolymerHydroxyethyl celluloseSurface tensionAqueous solution

Abstract

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Steady-shear rheology and surface activity of surfactant–polymer solutions were investigated experimentally. Four different polymers were studied as follows: cationic hydroxyethyl cellulose, nonionic hydroxyethyl cellulose, nonionic guar gum, and anionic xanthan gum. The influence of the following four surfactants on each of the polymers was determined: nonionic alcohol ethoxylate, anionic sodium lauryl sulfate, cationic hexadecyltrimethylammonium bromide, and zwitterionic cetyl betaine. The interaction between cationic hydroxyethyl cellulose and anionic sodium lauryl sulfate was extraordinarily strong, resulting in dramatic changes in rheological and surface-active properties. The consistency increased initially, reached a maximum value, and then fell off with the further addition of surfactant. The surface tension of surfactant–polymer solution dropped substantially and exhibited a minimum value. Thus, the surfactant–polymer solutions were much more surface-active compared with pure surfactant solutions. The interaction between anionic xanthan gum and cationic hexadecyltrimethylammonium bromide was also strong, resulting in a substantial decrease in consistency. The surfactant–polymer solution became less surface-active compared with pure surfactant solution due to the migration of surfactant from solution to polymer. The interactions between other polymers and surfactants were weak to moderate, resulting in small to modest changes in rheological and surface-active properties. Surface activity of surfactant–polymer solutions often increased due to the formation of complexes more surface-active than pure surfactant molecules.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.236
Threshold uncertainty score0.354

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.221
Teacher spread0.212 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it