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Record W4414566616 · doi:10.1021/acsanm.5c03473

Photoluminescence Enhancement at Telecom Wavelengths from PbS/CdS Quantum Dots coupled to a Plasmonic Crescent Metasurface

2025· article· en· W4414566616 on OpenAlexaff
Areeg Al-hamadani, Vaibhav Gupta, José Luis Montaño‐Priede, Rijil Thomas, Alina Muravitskaya, Laurent Markey, Céline Byl, Thomas Pons, Mario Zapata-Herrera, Nerea Zabala, Jean-Claude Weeber, Stephan Suckow, Nicolas Vogel, Jean‐Sebastien G. Bouillard, Ali M. Adawi

Bibliographic record

VenueACS Applied Nano Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicQuantum Dots Synthesis And Properties
Canadian institutionsInstitute of Particle Physics
FundersCentre National de la Recherche ScientifiqueEuropean Regional Development FundHorizon 2020 Framework ProgrammeEusko JaurlaritzaMinisterio de Ciencia, Tecnología e Innovación ProductivaIkerbasque, Basque Foundation for ScienceUniversity of Hull
KeywordsPlasmonPhotoluminescenceNanophotonicsQuantum dotPolarization (electrochemistry)WavelengthExcitation

Abstract

fetched live from OpenAlex

Efficient near-infrared (NIR) light sources are essential for a wide range of applications such as telecommunications, optoelectronic devices, biomedical sciences, infrared imaging, and machine vision. Colloidal quantum dots (QDs) have emerged as a promising platform for NIR technologies due to their tunable optical properties across the NIR spectrum, compatibility with silicon-based technology infrastructure, and ease of large-scale integration into nanophotonic systems. Coupling colloidal QDs with plasmonic structures provides an enhanced control over their optical properties. In this work, we investigate the coupling of a gold plasmonic crescent metasurface with NIR-emitting colloidal PbS/CdS QDs, at the telecommunication wavelength of 1.55 μm. The metasurface was specifically designed to allow for the selective excitation photoluminescence (PL) enhancement with polarization control, capitalizing on the anisotropic nature of the plasmonic crescents. Maximum PL enhancement factors of 1.6 were observed, with a strong dependence on the excitation wavelength and polarization. These findings, supported by full-wave three-dimensional finite-difference-time-domain (FDTD) numerical simulations, offer strategies to control and optimize the performance of colloidal QD-based NIR light sources for a wide range of applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0060.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.237
Teacher spread0.224 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes1
Has abstractyes

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