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Record W4414589503 · doi:10.1021/acs.cgd.5c00639

Lessons from Nature’s Freeze Crystallization-Perennial Sea Ice as a Model for Efficient Salt Rejection in Desalination

2025· article· en· W4414589503 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueCrystal Growth & Design · 2025
Typearticle
Languageen
FieldEngineering
TopicFreezing and Crystallization Processes
Canadian institutionsFuture Earth
Fundersnot available
KeywordsBrineDesalinationLow-temperature thermal desalinationCrystallizationSupercoolingSeawaterUltrapure waterOsmotic powerWork (physics)Solar energy

Abstract

fetched live from OpenAlex

Desalination remains essential for combating global water scarcity, yet conventional thermal and membrane methods are fundamentally constrained by excessive energy demands, operational complexity, and environmental trade-offs. Inspired by natural salt expulsion in perennial sea ice, this work revolutionizes freeze-melt desalination (FMD) by establishing nano/micron-scale ice crystallization kinetics as the critical determinant of ultrapure water yield. We demonstrate that a quasi-comb-shaped columnar saltwater ice (qCSCSI) microstructure, featuring orthogonally aligned brine channels within horizonal c -axis monocrystalline ice, drives spontaneous solute rejection via curvature-dominated interfacial thermodynamics. Submicron ice-front control ( r < 1 μm) minimizes brine trapping through synergistic Gibbs–Thomson confinement (Γ ≈ 29.7 K μm), ultralow interfacial viscosity (η eff ≪ 1 mPa s), and kinetic supercooling dynamics (Δ T > −0.014 K), synergistically optimizing growth velocities ( v n < 263 μm/s) for maximal salt rejection. Resolving FMD’s energy bottleneck, ambient cold harvesting transforms system energetics: polar qCSCSI-FMD leverages cryospheric cycles (specific consumption ≈ 20.06 kWh/m 3 ), while nonpolar designs exploit radiative/convective cooling inspired by cave ice formations. This dual innovation, bioinspired crystallization control coupled with passive cryogenic energy utilization, eliminates energy-intensive refrigeration and mechanical separation requirements, establishing qCSCSI-FMD as a scalable, low-carbon solution closing the water-energy nexus for sustainable security.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.951
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.257
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it