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Record W4414715985 · doi:10.1080/00084433.2025.2566580

An investigation into the role of alkaline scrubbing in spodumene flotation using X-Ray Absorption Near-Edge Structure (XANES) spectroscopy

2025· article· en· W4414715985 on OpenAlexafffund
Brian Kawenski Cook, K.O. Beatty, Luke Woolcock, Lucia Zuin, Charlotte E. Gibson

Bibliographic record

VenueCanadian Metallurgical Quarterly · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMinerals Flotation and Separation Techniques
Canadian institutionsCanadian Light Source (Canada)SGS (Canada)Queen's University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsData scrubbingAbsorption (acoustics)SpectroscopySpodumeneAbsorption spectroscopyAdsorption

Abstract

fetched live from OpenAlex

Spodumene is an important lithium aluminosilicate mineral in the battery supply chain found alongside other silicates with similar surface properties. It can be selectively concentrated by flotation using fatty acid collectors. Historic and modern research has shown how alkaline scrubbing improves spodumene flotation performance, however, its application is inconsistent. This study presents the first use of X-Ray Absorption Near-Edge Structure (XANES) Total Fluorescence Yield (FLY) spectra at the Li K-edge and Al L2,3 edge to evaluate sodium hydroxide treatments of four different spodumene samples. The findings confirmed the spodumene XANES spectra was consistent across all samples and suggested a continuous shift to lower energy occurred along the Li K-edge after alkaline scrubbing, in addition to potential cyclical shifts in peak energy along the Al L2,3 edge. Observed peak shifts were attributed to broken Al–O and Si–O bonds on the spodumene surface. Corresponding batch flotation results revealed selectivity and recovery were improved after scrubbing, with a greater observed improvement for a ‘weathered’ ore. This study demonstrates the potential use of XANES spectroscopy in lithium flotation research and provides further evidence that NaOH scrubbing is beneficial for spodumene flotation performance and should be considered as an integral part of spodumene flotation flowsheets.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.903
Threshold uncertainty score0.894

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.250
Teacher spread0.243 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

Explore more

Same venueCanadian Metallurgical QuarterlySame topicMinerals Flotation and Separation TechniquesFrench-language works237,207