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Record W4414740787 · doi:10.1093/clinchem/hvaf086.662

B-275 The Evolving Illicit Opioid Landscape: Insights into Fentanyl Analogs Para-Fluorofentanyl and Ortho-Methylfentanyl

2025· article· en· W4414740787 on OpenAlexaff
Melissa J. Bennett, David W. Kinniburgh

Bibliographic record

VenueClinical Chemistry · 2025
Typearticle
Languageen
FieldMedicine
TopicOpioid Use Disorder Treatment
Canadian institutionsPolicyWise for Children & Families
Fundersnot available
KeywordsFentanylUrineImmunoassayDrugOpioidIllicit drugPotency

Abstract

fetched live from OpenAlex

Abstract Background The illicit drug landscape has shifted significantly with changes in the availability, use and types of novel psychoactive substances. Two such substances, para-fluorofentanyl (pFF) and ortho-methylfentanyl (OMF), illicit fentanyl analogs, have increasingly surfaced in recent years. Their potency varies across different drug supplies due to the unregulated and clandestine nature of their chemical manufacturing process. This can pose a serious risk to users, as it can increase the likelihood of overdose and fatalities. Despite their presence, there remains a substantial gap in understanding these synthetic fentanyl analogs. This study aims to characterize the prevalence, concentration levels, and co-occurrence of pFF and OMF in urine samples from individuals dependent on opioids. Additionally, it seeks to evaluate the cross-reactivities of these substances with a fentanyl immunoassay. Methods Urine samples were collected and analyzed over an eight-month period for fentanyl, norfentanyl, and pFF, while OMF testing was conducted on samples collected over three months. Immunoassay data was obtained using an Olympus AU480 instrument with the Thermo Scientific DRI Fentanyl assay. Mass spectrometry analysis was performed using an internally developed dynamic multiple reaction monitoring method on an Agilent 6470 triple quadrupole instrument. To assess cross-reactivity, OMF was spiked into urine in triplicate at concentrations of 1, 2, 5, 10, 20, 50, 100, 200, and 500 ng/mL, while pFF was tested at 1, 2, 3, 5, and 10 ng/mL. Results Over an eight-month period, a total of 4,808 urine samples underwent drug testing. Among these, 26% confirmed positive for fentanyl. We then examined the presence of fentanyl analogs, pFF and OMF in the fentanyl positive samples. During this period, 1,267 fentanyl-confirmed samples were analyzed, with 89% testing positive for pFF. pFF concentrations ranged from 2 to 7,300 ng/mL, with an average of 697 ng/mL. Since OMF was introduced later in our testing panel, we analyzed three months of data, totaling 528 fentanyl-confirmed samples. Of these, 75% tested positive for OMF, with concentrations ranging from 1 to 8,600 ng/mL with an average of 242 ng/mL. Among pFF-positive samples, 84% were also positive for fentanyl, 97% for norfentanyl, and 91% for OMF. In OMF-positive samples, 92% tested positive for fentanyl, 98% for norfentanyl, and 72% for pFF. Cross-reactivity analysis showed that pFF had a 41% cross-reactivity with the fentanyl immunoassay, while OMF exhibited minimal cross-reactivity (<2%). Conclusion Our findings highlight the widespread presence of fentanyl analogs in opioid-dependent populations, with pFF and OMF frequently co-occurring with fentanyl. Their high prevalence suggests significant distribution within the illicit drug supply. Cross-reactivity analysis revealed that pFF exhibits moderate immunoassay cross-reactivity, while OMF demonstrates minimal cross-reactivity, underscoring the need for confirmatory mass spectrometry testing. These results reinforce the evolving nature of the illicit opioid landscape and the necessity for continued monitoring and improved detection strategies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.177
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.343
Teacher spread0.325 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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