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Record W4414757524 · doi:10.1021/acs.jproteome.5c00435

mzPeak: Designing a Scalable, Interoperable, and Future-Ready Mass Spectrometry Data Format

2025· review· en· W4414757524 on OpenAlexafffund
Tim Van Den Bossche, Theodore Alexandrov, Aivett Bilbao Pena, Wout Bittremieux, Federico Iván Brigante, Matthew Chambers, Joshua Charkow, Eric W. Deutsch, Andrew W. Dowsey, Yasin El Abiead, Ralf Gabriels, Helge Hecht, Steffen Heuckeroth, Joshua Klein, Michael D. Knierman, Lennart Martens, Robert L. Moritz, Laura‐Isobel McCall, Steffen Neumann, Yasset Pérez‐Riverol, Hannes Röst, Elliott J. Price, Jim Shofstahl, David L. Tabb, Julian Uszkoreit, Juan Antonio Vizcaíno, Mingxun Wang, Sander Willems, Dirk Winkelhardt, Oliver Kohlbacher, Samuel Wein

Bibliographic record

VenueJournal of Proteome Research · 2025
Typereview
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicMetabolomics and Mass Spectrometry Studies
Canadian institutionsUniversity of Toronto
FundersBiotechnology and Biological Sciences Research CouncilEngineering and Physical Sciences Research CouncilMinisterium für Wissenschaft, Forschung und Kunst Baden-WürttembergDeutsche ForschungsgemeinschaftEuropean Bioinformatics InstituteFonds Wetenschappelijk OnderzoekSilicon Valley Community FoundationNational Institute of Allergy and Infectious DiseasesChan Zuckerberg InitiativeWellcome TrustNational Institute of General Medical SciencesOffice of the DirectorBundesministerium für Bildung und ForschungBurroughs Wellcome FundNational Institutes of HealthCanadian Institutes of Health ResearchNational Science Foundation
KeywordsInteroperabilityMetadataWorkflowFile formatData formatVolume (thermodynamics)Mass spectrometryData curationData access

Abstract

fetched live from OpenAlex

Advances in mass spectrometry (MS) instrumentation, including higher resolution, faster scan speeds, and improved sensitivity, have dramatically increased the data volume and complexity. The adoption of imaging and ion mobility further amplifies these challenges in proteomics, metabolomics, and lipidomics. Current open formats such as mzML and imzML struggle to keep pace due to large file sizes, slow data access, and limited metadata support. Vendor-specific formats offer faster access but lack interoperability and long-term archival guarantees. We here lay the groundwork for mzPeak, a next-generation community data format designed to address these challenges and support high-throughput, multidimensional MS workflows. By adopting a hybrid model that combines efficient binary storage for numerical data and both human- and machine-readable metadata storage, mzPeak will reduce file sizes, accelerate data access, and offer a scalable, adaptable solution for evolving MS technologies. For researchers, mzPeak will support complex workflows and regulatory compliance through faster access, improved metadata, and interoperability. For vendors, it offers a streamlined, open alternative to proprietary formats. mzPeak aims to become a cornerstone of MS data management, enabling sustainable, high-performance solutions for future data types and fostering collaboration across the mass spectrometry community.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.006
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.946
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0060.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0020.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0020.002
Research integrity0.0000.002
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.124
GPT teacher head0.428
Teacher spread0.304 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes2
Has abstractyes

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