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Record W4414863312 · doi:10.26434/chemrxiv-2025-vrlkc

Atomically-thin Two-dimensional π-conjugated Kagomé Polymer with Dirac Cone-Driven Charge Transport

2025· preprint· en· W4414863312 on OpenAlexaff
Dominik Dettmann, Alessandro Pecchia, A. Notargiacomo, Marialilia Pea, Stefano Franchi, Michele Re Fiorentin, Ehsan Hamzehpoor, Aleksandar Mikov, Navathej Preetha Genesh, Gianluca Galeotti, Barbara Paci, Tarnjit Kaur Johal, Valerio Di Palma, M. Fanciulli, A. Sgarlata, Maurizia Palummo, Emanuele Orgiu, Federico Rosei, G. Contini

Bibliographic record

VenueChemRxiv · 2025
Typepreprint
Languageen
FieldPhysics and Astronomy
TopicTopological Materials and Phenomena
Canadian institutionsMcGill UniversityUniversité de MontréalUniversité du Québec à MontréalInstitut National de la Recherche Scientifique
Fundersnot available
KeywordsNanoelectronicsAmbipolar diffusionDensity functional theoryAb initioLattice (music)Electronic band structureElectronic structureDirac (video compression format)Ohmic contactSymmetry (geometry)

Abstract

fetched live from OpenAlex

Two-dimensional nanomaterials are at the forefront of next-generation technologies, with applications spanning quantum computing, catalysis, and sensing. Among these, on-surface synthesized two-dimensional conjugated polymers (2DCPs) with kagomé lattice symmetry have recently emerged as promising candidates, thanks to their ability to form large, ordered domains and their unique electronic structures featuring both flat bands and Dirac cones. In this work, we report the integration of atomically-thin, surface-confined 2DCPs into field-effect transistors (FETs), marking a step toward their use in functional devices. The fabricated FETs exhibit ohmic transport behavior with Pt contacts and reveal ambipolar graphene-like field induced conductivity modulation, directly linked to the Dirac cone in the electronic band structure. These findings are supported by ab initio density functional theory (DFT) calculations and finite element simulations of the drift-diffusion equation, confirming the transport characteristics. Our results highlight the potential of 2DCPs with kagomé lattice symmetry as highly tunable, organic systems for future applications in nanoelectronics and high-performance sensing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.238
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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