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Record W4415173650 · doi:10.1029/2025gl116033

Summertime Diurnal Variability of Formaldehyde Over the Contiguous United States: Constraints From Pandonia Global Network

2025· article· en· W4415173650 on OpenAlexaff
Tianlang Zhao, Jingqiu Mao, Xiaoyi Zhao, Apoorva Pandey, Viral Shah, K. Emma Knowland, Jennifer Kaiser, Martin Tiefengraber, Manuel Gebetsberger, Alexander Cede, Elena Spinei, T. F. Hanisco

Bibliographic record

VenueGeophysical Research Letters · 2025
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsEnvironment and Climate Change Canada
FundersNuclear Safety and Security CommissionOffice of Experimental Program to Stimulate Competitive ResearchLangley Research CenterNational Aeronautics and Space Administration
KeywordsTroposphereDiurnal cycleDiurnal temperature variationPlanetary boundary layerOzone Monitoring InstrumentGeostationary orbitSatelliteFormaldehydeTropospheric ozone

Abstract

fetched live from OpenAlex

Abstract The diurnal cycle of Formaldehyde (HCHO) provide critical insights into tropospheric photochemistry. Here we use tropospheric HCHO retrievals from the Pandonia Global Network (PGN), combined with NASA's GEOS Composition Forecast (GEOS‐CF) model to understand the diurnal variation of summertime HCHO across the contiguous US. While PGN HCHO tropospheric column (HCHO trop ) shows a weak diurnal cycle in most regions, a distinct midday peak is found at the urban sites of Southern US (mainly in Houston), likely driven by highly reactive VOC emissions. For the vertical profile of HCHO mixing ratio within the Planetary Boundary Layer (PBL), PGN shows a significant decrease from 0.5 to 2 km while GEOS‐CF exhibits an excessively well‐mixed vertical shape. This discrepancy in HCHO profile leads to an overestimated HCHO trop in GEOS‐CF in Northeast Coastal US and Southeast US. These findings offer valuable insights for interpreting geostationary satellite observations and understanding model biases in surface ozone (O 3 ).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.196
Threshold uncertainty score0.389

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.279
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes1
Has abstractyes

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