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Record W4415612457 · doi:10.1016/j.jwpe.2025.108914

Development and experimental validation of a mathematical model for fluoride-removal filters comprising chemically treated mineral rich carbon

2025· article· en· W4415612457 on OpenAlexaff
Lucy C. Auton, Shanmuk Srinivas Ravuru, Sirshendu De, T.G. Myers, Abel Valverde

Bibliographic record

VenueJournal of Water Process Engineering · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicFluoride Effects and Removal
Canadian institutionsUniversity of Alberta
FundersMinisterio de UniversidadesAgencia Estatal de InvestigaciónMinisterio de Ciencia e InnovaciónGeneralitat de CatalunyaEuropean Regional Development FundUniversity of Oxford
KeywordsFluorideInterpretabilityAdsorptionCarbon fibersFilter (signal processing)Robustness (evolution)Inlet

Abstract

fetched live from OpenAlex

Excessive fluoride intake can lead to dental and skeletal fluorosis, among other health issues. Naturally occurring fluoride and industrial runoff can result in concentrations far exceeding the World Health Organization’s recommended limits in water supplies. In this study, we derive a model incorporating the dominant mechanisms governing fluoride removal from drinking water using the two adsorbents mineral-rich carbon (MRC) and chemically treated mineral-rich carbon (TMRC). Using both new and previously published experimental data, we validate the model for MRC, TMRC, and their mixture, using both batch and column data. Despite the filters containing approximately 40:1 MRC:TMRC ratio by mass, we find that TMRC dominates fluoride removal, while MRC contributes at early and late times. The full column model, which uses parameters from isotherm batch studies, achieves excellent agreement with experimental breakthrough data across varying inlet concentrations and flow rates (R 2 > 0 . 991 , SSE < 0 . 0632 ). Motivated by this, we propose a reduced model based solely on TMRC adsorption, with a single fitting parameter, which still performs well across all breakthrough curves (R 2 > 0 . 983 , SSE < 0 . 117 ). The simplicity of this model means that it is straightforward and inexpensive to work with numerically. In both models, batch and column behaviours are reconciled and, for the case of breakthrough curves with varying inlet concentrations, a set of globally optimised parameters is found. The strong agreement with experimental data supports the model’s robustness and reinforces the physical interpretability of its parameters. These models for MRC and TMRC provide a foundation for filter optimisation and future efforts aimed at improving fluoride removal in resource-limited settings.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.200
Threshold uncertainty score0.320

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.226
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes1
Has abstractyes

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