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Record W4415647227 · doi:10.26434/chemrxiv-2025-fz6x8

The MassBank contributions of the mFam Consortium

2025· preprint· en· W4415647227 on OpenAlexaff
Anusha Ahlendorf, Khabat Vahabi, Tillmann G. Fischer, Pierre‐Marie Allard, Megan M. Augustin, Ulschan Bathe, David Broadhurst, Corey D. Broeckling, Joerg M. Buescher, Katyeny Manuela da Silva, Ric C. H. de Vos, Stefanie Döll, Maximilian Frey, Emmanuel Gaquerel, Vasuk Gautam, Alain Goossens, Jérémy Grosjean, Maria Halabalaki, Elias Iturrospe, Kim Kultima, Stephanie Herman, Toni M. Kutchan, Romain Larbat, Tytus D. Mak, René Meier, Eleni V. Mikropoulou, Grégory Mouille, Luca Nicolotti, François Perreau, Pierre Pétriacq, Michael Reichelt, Stacey N. Reinke, Rani Robeyns, Amy M. Sheflin, Alena Soboleva, Otmar Spring, Akshai Parakkal Sreenivasan, Jean Chrisologue Totozafy, Hiroshi Tsugawa, Josep Valls, Maria van de Lavoir, Justin J. J. van der Hooft, Fredd Vergara, David S. Wishart, Ludger A. Wessjohann, Jean‐Luc Wolfender, Jörg Ziegler, Gerd Ulrich Balcke, Steffen Neumann

Bibliographic record

VenueChemRxiv · 2025
Typepreprint
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicMetabolomics and Mass Spectrometry Studies
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsIdentification (biology)MetadataAnnotationMetabolomicsMetaboliteResource (disambiguation)

Abstract

fetched live from OpenAlex

The analysis of metabolic profiles using high resolution mass spectrometry (MS) data gives deep insights into the biological processes. In metabolomics, MS generates a large number of features that represent metabolites. However, identifying specific metabolites from these features can be challenging. One of the major bottlenecks in the metabolomics field is the identification of MS features, which is a prerequisite for any biochemical interpretation. By identifying similarities and differences within a family, evaluating MS features at the metabolite family level can help assign functional roles to individual MS features. This data can help interpret metabolic pathways and processes within a biological system. For the assignment of metabolite families to MS features, it is very important to have good quality, reliable, and diverse spectral libraries. We initiated a global effort to collect high-resolution MS/MS spectra of metabolites from all biological origins, including mammals, microorganisms, and plants. The mFAM-MS/MS Collection delivers valuable training data to assign machine-readable classified information on the unknown metabolites. The mFam Consortium used a standardized metadata template and has developed a globally curated MS/MS spectral library of 7,872 spectra with 2,126 unique metabolites. This library was compiled from 47 datasets contributed by 25 laboratories and leverages 12 instrument types, including QTOF, Orbitrap, and Ion Mobility systems. It comprises 4,646 spectra in positive mode and 3,226 in negative mode. This standardized resource significantly enhances metabolite identification capabilities, supports the development of machine learning-based annotation tools, and accelerates the discovery of novel metabolites. All spectra are available under the collective contributor label mFam in the MassBank system, including the web interface and the 2025.10 data release available at GitHub and Zenodo.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.009
metaresearch head score (Gemma)0.026
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Dataset · Consensus signal: none
Teacher disagreement score0.097
Threshold uncertainty score0.325

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0090.026
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0110.012
Science and technology studies0.0030.001
Scholarly communication0.0080.010
Open science0.0040.009
Research integrity0.0030.003
Insufficient payload (model declined to judge)0.0970.095

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.263
Teacher spread0.254 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreDataset

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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