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Record W4415701345 · doi:10.1021/acs.jced.5c00421

Round Robin Measurements of Molten Salt Properties for LiF-NaF-KF (FLiNaK) and NaCl-KCl Mixtures

2025· article· en· W4415701345 on OpenAlexafffund
Troy Munro, Randall Chiu, Melissa A. Rose, Ondřej Beneš, Miroslav Boča, D. Nathanael Gardner, Amanda Leong, Sara Mastromarino, Kim L. Pamplin, M.H.A. Piro, Mouna Saoudi, Juliano Schorne‐Pinto, Christian Michael Sclafani, Anna L. Smith, Nathan D. Smith, Dino Sulejmanovic, Allison M. Berry, Renkun Chen, Ka Man Chung, Christa Dahman, Kent P. Detrick, Tianshi Feng, Jaén A. Ocádiz Flores, Ryan Gallagher, Levi Gardner, Xiaofeng Guo, Jay Matthew Jackson, Toni Karlsson, Peter Kasper, Hojong Kim, Logan J McIlwain, Matthew Memmott, Brian Merritt, Marisa J. Monreal, K Oishi, L. V. Orlovskaya, Stephen Parker, Andrew A. Prudil, Aaron D. Robison, Sean Scott, John Vlieland, Michael E. Woods, Jinsuo Zhang, Theodore M. Besmann, Raluca O. Scarlat

Bibliographic record

VenueJournal of Chemical & Engineering Data · 2025
Typearticle
Languageen
FieldChemical Engineering
TopicMolten salt chemistry and electrochemical processes
Canadian institutionsPolytechnique MontréalCanadian Nuclear LaboratoriesMcMaster University
FundersNational Science Foundation Graduate Research Fellowship ProgramOak Ridge National LaboratoryLaboratory Directed Research and DevelopmentCanadian Nuclear LaboratoriesSolar Energy Technologies OfficeOntario Power GenerationNatural Sciences and Engineering Research Council of CanadaLos Alamos National LaboratoryAtomic Energy of Canada LimitedArgonne National LaboratoryU.S. Department of EnergyUniversity of Ontario Institute of TechnologyU.S. Nuclear Regulatory CommissionNuclear Energy University ProgramCanada Foundation for InnovationOntario Ministry of Economic Development, Job Creation and Trade
KeywordsMolten saltSalt (chemistry)HalideWork (physics)ThermalRound robin testProperty (philosophy)

Abstract

fetched live from OpenAlex

The development, operation, and regulation of nuclear reactors that utilize molten salts as fuel or as heat transfer media require knowledge of the thermal properties of the salt systems and quantification of the corresponding uncertainties. Knowledge of molten salt properties is also necessary for applications in material synthesis, processing, separations, solar thermal power generation, and energy storage. A round robin was conducted with national laboratory and university participants from twenty-one laboratories in five countries to compare property measurements, to better understand uncertainties, and to identify possible best practices. Two salt mixtures, each from a common batch, were distributed to participants for evaluation: equimolar NaCl-KCl and 45.0LiF-13.7NaF-41.3KF mol % (FLiNaK). Measurements were performed to determine the major constituent composition, oxygen content, density, thermal expansivity, melting point, and thermal conductivity. Error analysis was performed on each measurement for uncertainty quantification for each type of property that was explored. The resulting discussion of the methodologies used in this work is meant to lay the groundwork for the development of standard methods and reference materials for future high-temperature property measurements on halide melts.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.083
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.269
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

Explore more

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