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Influence of residence time on the particle-gas partitioning of phthalates onto airborne inorganic particle

2025· article· en· W4415942995 on OpenAlexafffund
Azad Bahrami, Fariborz Haghighat, Jiping Zhu

Bibliographic record

VenueAtmospheric Environment · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicEffects and risks of endocrine disrupting chemicals
Canadian institutionsHealth CanadaConcordia University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPhthalateParticulatesIndoor air qualityDilutionResidence time (fluid dynamics)Particle (ecology)Diethyl phthalateParticle number

Abstract

fetched live from OpenAlex

In indoor environments, the presence of particulate matter promotes SVOCs volatilization, increasing their overall concentration in the air. This effect arises from the partition of SVOCs between the gas and particulate phases. The particle-gas partition ratio ( K p ) is a critical parameter influencing the fate, transport, and human exposure to indoor SVOCs. Air exchange rate (AER) is a pivotal factor in closed spaces as it regulates the residence time of airborne SVOCs in an indoor environment. It has been reported that AER (or residence time) can affect particle-gas partitioning behavior for organic particles when equilibrium between gas and particle phases is not reached; however, its effect on inorganic particles has not been thoroughly investigated. This study develops an experimental procedure to measure K p of Di-n-butyl phthalate (DnBP) and Diethyl phthalate (DEP) with inorganic sodium chloride (NaCl) particles. Results shows that DnBP had higher K p values than DEP. Positive correlation of K p values and mixing time was observed. These findings are consistent with model predictions. Further experiments were carried out to study the impact of AER on K p , and the results shown that higher air exchange rates (lower residence time) result in lower particle-phase concentrations of SVOCs due to increased dilution and reduced interaction time with particles. These findings have important implications for indoor air quality assessments, highlighting the influence of ventilation strategies on SVOCs behavior in indoor environments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.148
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.250
Teacher spread0.245 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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