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Record W4415958665 · doi:10.1021/acs.jpclett.5c01792

Revisiting the Shockley–Queisser Limit: Understanding Solar Cell Efficiency in One Sun and Indoor Environments

2025· article· en· W4415958665 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueThe Journal of Physical Chemistry Letters · 2025
Typearticle
Languageen
FieldEngineering
Topicsolar cell performance optimization
Canadian institutionsToronto Metropolitan University
FundersNational Research Foundation of Korea
KeywordsIncandescent light bulbBlack-body radiationPhotovoltaic systemLight-emitting diodeLimit (mathematics)Radiative transferTransmittanceEnclosure

Abstract

fetched live from OpenAlex

junction as a blackbody (BB) illuminated by the sun as a BB, remains a theoretical benchmark but overlooks key loss mechanisms like nonradiative recombination. By reproducing the SQL and incorporating the external radiative efficiency (ERE), we quantify real-world efficiency losses. Our findings show that GaAs and perovskite solar cells, with minimal nonradiative losses, approach theoretical limits under both AM1.5G and indoor lighting. We also demonstrate that BB intensity─modulated by temperature or geometric factors─shifts optimal efficiency: lower BB temperatures cause a red shift, while reduced geometric factors induce a blue shift. Among artificial sources, LEDs and fluorescents offer the best performance at higher energies, whereas incandescent light favors lower energies. These results highlight the need to minimize nonradiative losses and tailor device design to specific spectral irradiance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.271
Threshold uncertainty score0.282

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.192
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it