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Record W4416008303 · doi:10.5194/acp-25-15077-2025

Transport of Biomass Burning Aerosol into the Extratropical Tropopause Region over Europe via Warm Conveyor Belt Uplift

2025· article· en· W4416008303 on OpenAlexaboutno aff
Philipp Joppe, Johannes Schneider, Jonas Wilsch, Heiko Bozem, Anna Breuninger, Joachim Curtius, M.-O. Ebert, Nicolas Emig, Peter Hoor, Sadath Ismayil, Konrad Kandler, Daniel Kunkel, Hans‐Christoph Lachnitt, Yun Li, Annette Miltenberger, Sarah Richter, Christian Rolf, Lisa Schneider, Cornelis Schwenk, Nicole Spelten, Alexander L. Vogel, Yafang Cheng, Stephan Borrmann

Bibliographic record

VenueAtmospheric chemistry and physics · 2025
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsnot available
FundersDeutsche Forschungsgemeinschaft
KeywordsAerosolTropopauseExtratropical cycloneTroposphereTrace gasRadiative transferStratosphereParticle (ecology)Mixing ratio

Abstract

fetched live from OpenAlex

We present measurements from the aircraft-based TPEx (Tropopause composition gradients and mixing Experiment) mission in June 2024 over Europe. The measurement platform, a Learjet 35A, was equipped with in-situ trace gas and aerosol measurements and filter samplers for offline analysis. For vertical gradient measurements of trace species and aerosol, we conducted redundant measurements on a fully automated towed sensor shuttle (TOSS) 200 m below the aircraft. On 17 June 2024, we observed a filament with elevated aerosol number concentrations of up to 800 particles cm −3 between 100 nm and 1 µm. This is higher by a factor of two to four than the local background. Carbon monoxide (CO) mixing ratios were larger than 100 ppbv. Single particle analysis of impactor samples using electron microscopy show characteristic biomass burning (BB) aerosol in the tropopause region. The TOSS measurements also allow the calculation of the potential temperature gradient (Δθ⋅Δz-1). Within the polluted filament, we observe changes towards smaller gradients, which is presumably due to an increase of potential temperature at lower altitudes by radiative heating as a consequence of the transported BB aerosol. Trajectory analysis show air mass origin over Canada with low-level long-range transport and subsequent uplift by a warm conveyor belt (WCB) over Europe as additional pathway of pollution into the UTLS. Furthermore, this analysis yields that BB aerosol can be transported in a WCB into the UTLS there it can be mixed with stratospheric air masses.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score0.134

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.204
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes1
Has abstractyes

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