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Record W4416023813 · doi:10.1111/1750-3841.70628

Behavior of Dissociated Salts in Aqueous Solution: Insights From T <sub>2</sub> Relaxation Time and Signal Intensity Using a LF‐NMR

2025· article· en· W4416023813 on OpenAlexafffund
Afroza Sultana, Ali Asghari, Christophe Cordella, Seddik Khalloufi

Bibliographic record

VenueJournal of Food Science · 2025
Typearticle
Languageen
FieldPhysics and Astronomy
TopicSpectroscopy and Quantum Chemical Studies
Canadian institutionsUniversité LavalAgriculture and Agri-Food Canada
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsAqueous solutionRelaxation (psychology)Chaotropic agentSalt (chemistry)RelaxometryIonic bondingEnthalpyDivalent

Abstract

fetched live from OpenAlex

ABSTRACT This study explores the influence of NaCl, KCl, CaCl 2 , and MgCl 2 , salts commonly used in the food industry, on aqueous solutions using transverse (T 2 ) relaxometry in low‐ field nuclear magnetic resonance (LF‐NMR) at a salt‐to‐water ratio ranging from 0 to 0.1079 mol/mol. The results demonstrate that T 2 relaxation times are significantly affected by the chemical nature and concentration of the ions, with divalent salts exhibiting distinct behavior compared to monovalent salts. Notably, the kosmotropic (structure‐making) and chaotropic (structure‐breaking) properties of the salts were found to influence relaxation times. Mg 2+ exhibited the most pronounced effect (low relaxation time) due to its high charge density and strong hydration ability, followed by Ca 2+ , Na + , and K + . Relaxation times decreased with increasing salt concentration for MgCl 2 , CaCl 2, and NaCl (from 3080 ms at 0% to 504, 1671, and 2796 ms at 0.1079 mol/mol, respectively), whereas the chaotropic KCl solution had extended relaxation times (3884 ms at 0.0771 mol/mol). A novel finding of this study is the exponential decay of peak area in salt solutions, as evidenced by experimental data. The alteration in the structural arrangement of water and the synergistic movement of cations or anions in higher‐mass salt solutions are hypothesized to underlie the observed behavior, although the exact reason requires further study. Electrical conductivity (EC), water activity, and the enthalpy of solution upon salt incorporation provide further insights into the behavior of salt solutions. This research advances the understanding of how ionic solutes modulate water dynamics, affecting both relaxation time and the total peak area.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.086
Threshold uncertainty score0.222

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.257
Teacher spread0.245 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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