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Record W4416411499 · doi:10.1021/acs.analchem.5c05475

Photoacoustic Spectroscopy Dual-Gas Sensor for CH <sub>4</sub> and NH <sub>3</sub> Based on Dual-Path Dense Spot Multipass Cell and Dual-Frequency Photoacoustic Cell

2025· article· en· W4416411499 on OpenAlexafffund
Chu Zhang, Ying He, Shunda Qiao, Lixian Liu, Andreas Mandelis, Yufei Ma

Bibliographic record

VenueAnalytical Chemistry · 2025
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsUniversity of Toronto
FundersHeilongjiang Provincial Postdoctoral Science FoundationNatural Science Foundation of Heilongjiang ProvinceChina Postdoctoral Science FoundationNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of China
KeywordsPhotoacoustic spectroscopyAmplifierPhotoacoustic imaging in biomedicinePhotoacoustic effectLaserSpectroscopyRaman spectroscopyDetection limitResonance (particle physics)

Abstract

fetched live from OpenAlex

In this paper, a highly sensitive methane (CH 4 ) and ammonia (NH 3 ) dual-gas photoacoustic spectroscopy (PAS) gas sensor based on a dual-path high-spot-density multipass cell (MPC) and dual-frequency photoacoustic cell (PAC) was demonstrated for the first time. A dual-path MPC mathematical model was established to achieve multiple independent rings and 223 excitations of dual gases. In order to integrate with the MPC more conveniently, the designed dual-frequency PAC was used to excite the Helmholtz resonance mode. A Raman fiber amplifier (RFA) and an erbium-doped fiber amplifier (EDFA) were employed to amplify the output power of the two diode lasers to enhance the excitation intensity. The experimental results indicated that when the output power was set as 50 and 300 mW, respectively, the 2 f signals for CH 4 and NH 3 detection with the high-spot-density MPC showed 41.91-fold and 41.30-fold enhancements compared to the system without MPC, demonstrating significant performance improvement. The minimum detection limits (MDLs) of CH 4 and NH 3 were found to be 65 and 374 ppb, respectively, when the average time of the CH 4 /NH 3 –PAS dual-gas sensor was 1000 s.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.124
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.240
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes2
Has abstractyes

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