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Hydrogels for Analyte Sensing

2025· article· en· W4416422967 on OpenAlexafffund
Katia Cherifi, Simon Matoori

Bibliographic record

VenueACS Measurement Science Au · 2025
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicHydrogels: synthesis, properties, applications
Canadian institutionsUniversité de Montréal
FundersFaculté de pharmacie, Université de Montréal
KeywordsSelf-healing hydrogelsAnalyteLeverage (statistics)MultiplexingOptical sensingNanoporousElectrical conductorOptical fiber

Abstract

fetched live from OpenAlex

Hydrogels have emerged as a versatile platform technology for analyte sensing, offering unique advantages in tunable chemistry, for loading with sensors across multiple length scales, and biocompatibility. These smart materials undergo predictable changes in optical properties, conductivity, swelling, and porosity upon analyte interaction, enabling their function as biosensors. While hydrogels can respond to a variety of stimuli, their responses are most effectively quantified through optical and electrical readouts, which enable direct, real-time, and quantitative sensing in complex biological fluids. Optical approaches leverage fluorescence, chemiluminescence, and colorimetry, whereas electrical approaches leverage conductive fillers or redox-active groups. Hybrid platforms integrate multiple readout mechanisms, enhancing sensitivity, robustness, and multiplexing capabilities. Many of these systems were validated in various biological matrices, such as interstitial fluid, sweat, and wound exudates. Beyond technical advances, we discuss translational challenges including selectivity, stability, nonreversibility, signal standardization, device portability, and regulatory approval, as well as emerging opportunities in coupling hydrogel sensors with artificial intelligence for improved data interpretation and clinical integration. Together, these developments position hydrogel-based diagnostics as promising candidates for next-generation, real-time, point-of-care biosensing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.083
Threshold uncertainty score0.447

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.045
GPT teacher head0.287
Teacher spread0.243 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

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