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Record W4416653375 · doi:10.1080/10408436.2025.2586529

Graphene synthesis via thermal plasma: a comprehensive review of key process parameters and outcomes

2025· article· en· W4416653375 on OpenAlexafffund
Reem Mahmoud, F. Gitzhofer, Nicolas Abatzoglou

Bibliographic record

VenueCritical reviews in solid state and materials sciences/CRC critical reviews in solid state and materials sciences · 2025
Typearticle
Languageen
FieldMedicine
TopicPlasma Applications and Diagnostics
Canadian institutionsUniversité de Sherbrooke
FundersMitacs
KeywordsProcess (computing)Key (lock)ThermalGrapheneThermal conductivity

Abstract

fetched live from OpenAlex

Thermal plasma provides several advantages for graphene synthesis, including high conversion efficiency and rapid, continuous production. Furthermore, it enables precise control over process parameters, resulting in the production of high-quality graphene with low defects, leading to its usage in diverse applications. Despite these advancements, the primary challenge remains the low production rate of graphene, which limits the scalability and commercial viability of the synthesis process. The gas-phase graphene synthesis process is significantly influenced by factors such as pressure, power, hydrocarbon feedstock type and flow rates, plasma gas composition, catalyst presence, quenching rate, and oxygen/hydrogen content. A wide range of carbon nanostructures (including graphene (Gr), graphite, carbon black (CB), carbon nanotubes (CNTs), and carbon nanohorns (CNHs)) can be produced by modulating these factors. This review systematically investigates the impact of the aforementioned parameters on graphene synthesis and the underlying reaction mechanisms. It demonstrates the critical role of carbon concentration, temperature, and residence time in influencing plasma chemistry, and consequently the graphene quality, with major implications for advancing graphene-based technologies. This review article contributes to the existing literature by providing a comprehensive overview of the state of the art in thermal plasma-based graphene synthesis.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.006
metaresearch head score (Gemma)0.012
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMetaresearch, Meta-epidemiology (narrow), Science and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.435
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0060.012
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0030.000
Bibliometrics0.0000.001
Science and technology studies0.0000.005
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.055
GPT teacher head0.413
Teacher spread0.358 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

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