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Record W4416706553 · doi:10.1093/bulcsj/uoaf114

Stoichiometric and catalytic degradation of SF6 with cobaltocene

2025· article· en· W4416706553 on OpenAlexfundno aff
Vanessa A. Béland, Nils Nöthling, Josep Cornellà

Bibliographic record

VenueBulletin of the Chemical Society of Japan · 2025
Typearticle
Languageen
FieldChemistry
TopicInorganic Fluorides and Related Compounds
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of CanadaDeutsche Forschungsgemeinschaft
KeywordsCobaltoceneHeteronuclear moleculeCatalysisStoichiometrySalt (chemistry)InfraredInfrared spectroscopyFluoride

Abstract

fetched live from OpenAlex

Abstract The controlled reduction of SF6 (25 °C, 1 bar) with cobaltocene results in the formation of the mixed salt [Cp2Co]2[SF5][F]. The salt can be characterized by solution and solid-state heteronuclear nuclear magnetic resonance and infrared spectroscopies and demonstrates a degree of mineralization of the S and F atoms when reacted with borosilicate glass. Although [Cp2Co]2[SF5][F] is highly reactive, the structure of the corresponding [Cp2Co][F] is also reported herein, thus providing structural evidence for the naked fluoride anion. The mild activation of SF6 by cobaltocene also permits its catalytic degradation using phosphines as terminal reductants.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score0.256

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.192
Teacher spread0.187 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes1
Has abstractyes

Explore more

Same venueBulletin of the Chemical Society of JapanSame topicInorganic Fluorides and Related CompoundsFrench-language works237,207