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Record W4416756123 · doi:10.1016/j.elspec.2025.147578

Applications of auger electron spectroscopy in the chemical state analysis of copper and its oxides

2025· article· en· W4416756123 on OpenAlexafffund
Jeffrey D. Henderson, Mohammad Sabeti, Xuejie Li, Na Wang, Mehran Behazin, Mark C. Biesinger, James J. Noël, S. Ramamurthy

Bibliographic record

VenueJournal of Electron Spectroscopy and Related Phenomena · 2025
Typearticle
Languageen
FieldMaterials Science
TopicElectron and X-Ray Spectroscopy Techniques
Canadian institutionsNuclear Waste Management OrganizationWestern University
FundersNatural Sciences and Engineering Research Council of CanadaNuclear Waste Management OrganizationCanada Foundation for InnovationOntario Research Foundation
KeywordsCopperAuger electron spectroscopyChemical stateElectron spectroscopyAnalytical Chemistry (journal)Spectroscopy

Abstract

fetched live from OpenAlex

Electron-induced Auger electron spectroscopy was successfully applied to differentiate copper species, such as metallic Cu, Cu 2 O, CuO, and Cu(OH) 2 . To do so, high-quality standard spectra were collected and their key parameters, including peak positions, widths, intensity ratios, and peak shapes, were examined to evaluate their effectiveness in chemical state identification. Average values and standard deviations were reported for each parameter. The results reveal sufficient spectral differences among Cu metal, Cu 2 O, CuO, and Cu(OH) 2 to enable chemical fingerprinting, though no single parameter provided information sufficient for accurate speciation. Instead, a combination of spectral features must be used to enable reliable identification of these species. This approach was successfully applied to identify the chemical states of oxide layers formed on two different copper samples. The results from the Auger analyses were consistent with those from XPS measurements. This methodology was also applied to determine the presence of Cu 2 O oxide inclusions in cold sprayed copper, and the results were consistent with previously published results from TEM, EELS, and electron diffraction studies. Compared to these techniques, Auger electron spectroscopy requires minimal sample preparation and offers high spatial and surface sensitivity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score0.991

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.281
Teacher spread0.277 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes2
Has abstractyes

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