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Record W4416936152 · doi:10.3389/fmats.2025.1714941

Microstructural engineering of high-content rubber asphalt via precision devulcanization for enhanced performance

2025· article· en· W4416936152 on OpenAlex
Meng Yang, Shuai Li, Xiaohong Guo, M.H. Pu, Chongyuan Li, Xu Ouyang, Shuang Wu, Chaozhe Jiang, Yukun Li, Hanqing Mao, Lei Zhong, A. Wenqian

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueFrontiers in Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicAsphalt Pavement Performance Evaluation
Canadian institutionsUniversity of Waterloo
FundersDepartment of Science and Technology of Inner Mongolia
KeywordsAsphaltNatural rubberRheologyCrumb rubberCreepStress (linguistics)

Abstract

fetched live from OpenAlex

Introduction The practical deployment of high-content rubberized asphalt is often hindered by its compromised workability and unstable performance. Moving beyond conventional devulcanization approaches, this study introduces an integrated strategy of interface-controlled devulcanization and microstructural tailoring to address these challenges. Methods A bespoke devulcanizing agent (RubberSynth-AP) was synthesized to promote selective scission of sulfur-based crosslinks and improve interfacial adhesion. Coupled with an optimized production process, this method allows the stable integration of crumb rubber at concentrations up to 30% by binder weight. Multi-scale rheological analyses—encompassing temperature sweeps, multiple stress creep recovery (MSCR), and linear amplitude sweep (LAS) tests—were employed. Results An optimum rubber content of 26% was identified, exhibiting a superior combination of properties: a failure temperature of 76.5 °C, 40% lower viscosity, 53.12% recovery rate, and enhanced fatigue resistance. Mechanistic analysis uncovered a microstructural evolution from a heterogeneous, stress-concentrating system to a homogeneous, elastic-network-dominated morphology. This structural improvement supported the adoption of a dense-graded AC-13 mixture design, achieving a remarkable dynamic stability of 3,850 cycles/mm. Economically and environmentally, this technique promotes the consumption of 18 tons of waste rubber per lane-kilometer with a cost reduction of approximately ¥17,000. Discussion Collectively, this study demonstrates that the interface-controlled devulcanization strategy enables the production of high-content rubberized asphalt (up to 30%) with superior and balanced rheological properties, overcoming the longstanding workability-performance trade-off. The findings provide a scientifically-grounded and economically viable solution for developing sustainable pavement materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.269
Threshold uncertainty score0.695

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.214
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it