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Record W4416987379 · doi:10.1021/acsami.5c16811

Tailoring Single Photon Sources in Hexagonal Boron Nitride via Chemical Vapor Deposition and Nanoscale Focused Ion Beam Milling

2025· article· en· W4416987379 on OpenAlexaff
Rachael Klaiss, Joshua Ziegler, David J. Miller, Kara M. Zappitelli, Kenji Watanabe, Takashi Taniguchi, Sai Krishna Narayanan, Pratibha Dev, Benjamín Alemán

Bibliographic record

VenueACS Applied Materials & Interfaces · 2025
Typearticle
Languageen
FieldMaterials Science
TopicDiamond and Carbon-based Materials Research
Canadian institutionsImpact
FundersDivision of Materials ResearchJapan Society for the Promotion of ScienceOffice of Multidisciplinary ActivitiesDivision of Civil, Mechanical and Manufacturing InnovationUniversity of Oregon
KeywordsFocused ion beamChemical vapor depositionFabricationNanocrystalline materialPhotonCommon emitterIon beamNitrideGallium nitride

Abstract

fetched live from OpenAlex

Emerging quantum information technologies demand robust, tunable, single photon sources. Solid-state single photon emitters (SPEs) in the two-dimensional material hexagonal boron nitride (hBN) offer unique advantages, including stability and integration potential, yet current fabrication methods lack precise control over the emitter placement and properties. In this work, we demonstrate a high-yield approach to patterning SPE arrays in hBN by combining focused ion beam (FIB) milling with chemical vapor deposition (CVD) of nanocrystalline graphitic carbon. Using statistical design and analysis of experiments, we systematically map a high-dimensional parameter space─spanning FIB exposure and CVD conditions─to identify the optimal regimes for SPE formation and tunability. Our method leverages widely available fabrication tools and provides critical insights into defect activation mechanisms, offering a scalable, reproducible path toward controllable quantum emitter synthesis. Beyond hBN, this approach opens the door to generating defect-based SPEs in other low-defect solid-state materials. The result is a practical and versatile platform for creating quantum light sources tailored for applications in communication, sensing, and computation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.236
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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