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Record W4417104566 · doi:10.1002/adma.202519259

Electronic Excitation‐Driven β‐Ga <sub>2</sub> O <sub>3</sub> Metastability Transformation and Self‐Organization Mechanism: β→κ/γ/δ Phases

2025· article· en· W4417104566 on OpenAlexaff
Xinqing Han, Yalin Li, Miguel L. Crespillo, Eva Zarkadoula, Yong Liu, Wenxiang Mu, Shijun Zhao, Peng Liu

Bibliographic record

VenueAdvanced Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicGa2O3 and related materials
Canadian institutionsInstitute of Particle Physics
FundersNational Natural Science Foundation of China
KeywordsMetastabilitySpinelMolecular dynamicsNanoscopic scaleAnisotropyLattice (music)OxideRelaxation (psychology)Phase (matter)

Abstract

fetched live from OpenAlex

Abstract Irradiation‐driven multiphase self‐organization presents emergent opportunities for the customization of nanoscale engineering properties, dynamically tuning strain‐field distributions and interfacial electronic structures. Responding to intense electronic excitation‐induced energy deposition, the dominant phase transformations, with varying Gibbs free energy , are confirmed as β → κ → γ → δ that are located in specific microregions for Gallium (III) oxide (Ga 2 O 3 ), as follows: (i) Surface‐localized interstitial accumulation under compressive stress triggers β → δ via semi‐coherent interface formation. (ii) Tensile stress within latent tracks drives vacancy‐mediated oxygen layer truncation (4/12 periodicity along ⟨0001⟩), stabilizing coherent 4H (ABCB) κ and 3C (ABC) β (ABC) interfaces through strain‐compensated octahedral distortion. (iii) Screw dislocation‐mediated lattice relaxation induces β → γ via cation disordering (Ga 3 ⁺ occupancy at β ‐interstitial sites), forming metastable spinel γ with mixed occupancy across 16d/8a Wyckoff sites. Irradiation‐driven β ‐Ga 2 O 3 → κ/γ/δ transitions, as mechanistically revealed via inelastic thermal spike (i‐TS) calculations and molecular dynamics simulations, induce defect‐mediated nonlinear photoresponse, critical for optoelectronic engineering.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.019
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.220
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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