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Record W4417303355 · doi:10.1016/j.jece.2025.120691

Advanced oxidation of tertiary wastewater micropollutants with nearly-zero contact time

2025· article· en· W4417303355 on OpenAlexafffund
Jaime F. Mata De la Vega, Kourosh Nasr Esfahani, Ted Mao, Paolo Roccaro, Beatrice Cantoni, Domenico Santoro

Bibliographic record

VenueJournal of environmental chemical engineering · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicAdvanced oxidation water treatment
Canadian institutionsWestern University
FundersNextGenerationEUConsejo de Ciencia y Tecnología del Estado de GuanajuatoNatural Sciences and Engineering Research Council of CanadaConsejo Nacional de Ciencia y TecnologíaEuropean Commission
KeywordsOzonePollutantNitriteWastewaterWater qualityWater treatmentMass transferSewage treatment

Abstract

fetched live from OpenAlex

Ozone is a powerful oxidant capable of degrading a wide range of contaminants, but its low mass transfer with conventional devices poses challenges for effective application in advanced oxidation processes and highly reactive matrices such as wastewater. This study evaluates the performance of MITO 3 X ® technology, a system designed to enhance ozone mass transfer and radical yields therefore optimizing the reactivity between pollutants and oxidative species with almost instantaneous contact time (<1 s). This research investigates MITO 3 X ® efficacy in degrading seven pollutants including Methylene blue (MB), 4-chlorobenzoic acid (pCBA), Caffeine (Caf), Acetaminophen (APAP), Ciprofloxacin (Cipro), Carbamazepine (CBZ), and Sulfamethoxazole (SMZ) as a function of water quality (high, medium, and low). Here, ‘high’ denotes dechlorinated, GAC-filtered water without added scavengers; ‘medium’ includes 5 mg. L⁻¹ nitrite (NaNO₂); and ‘low’ includes both 5 mg. L⁻¹ nitrite and 10 mg. L⁻¹ TOC (as methanol) thereby reflecting progressively stronger radical/ozone-scavenging matrices. Results indicate that ozonation efficiency, measured as (C₀-C)/C₀*100, reached up to 85 ± 5 % under high water quality, and approximately 65 % in medium quality, and 45 % in low quality, highlighting the impact of scavengers on advanced oxidation performance. A multivariate analysis examined the effects of MITO 3 X ® operational parameters, including impeller speed, water flow rate, and ozone capacity, on pollutant removal. The mass of ozone injected (e.g., controlled via adjustment of ozone capacity of the ozone generator) was dominant, with mixing and water quality also contributing through their interactions. The results defined operating conditions that maximize removal under nearly zero (e.g., < 1 s) contact time and highlighted the potential of MITO₃X® as a compact, efficient ozonation option for tertiary wastewater treatment and micropollutant control.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score0.539

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.001
GPT teacher head0.168
Teacher spread0.167 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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