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Record W4417357375 · doi:10.26434/chemrxiv-2025-dhdmn

Dual-Function Metal–Phenolic Networks-Capped Starch Nanoparticles for Postharvest Pesticide Removal and Produce Preservation

2025· article· W4417357375 on OpenAlexaff
Tang Jin, Zhangmin Wan, Ivy Chiu, Yan Song, Gary Othniel Wijaya, Orlando J. Rojas, Keng C. Chou, Rickey Y. Yada, Tianxi Yang

Bibliographic record

VenueChemRxiv · 2025
Typearticle
Language
FieldMaterials Science
TopicNanocomposite Films for Food Packaging
Canadian institutionsUniversity of British Columbia
Fundersnot available
KeywordsPostharvestPesticide residuePesticideStarchTitratable acidCoatingPolyphenol

Abstract

fetched live from OpenAlex

The safety and quality of fresh produce are increasingly challenged by pesticide residues and postharvest losses. Traditional postharvest treatments often show limited effectiveness in removing pesticide residues and may introduce micro/nanoplastics contaminations, leading to the need for innovative solutions that both enhance pesticide removal and preserve produce quality. Herein, we developed a novel dual-function postharvest wash based on metal–phenolic networks capped-starch nanoparticles (FTN@SNPs), designed to synergistically remove pesticide residues and reduce postharvest deterioration. The wash formulation integrates the nutritive polyphenol tannic acid and iron ions into a metal–phenolic networks (MPNs), which is further capped onto starch nanoparticles to create a multifunctional solution with effective washing capability, antimicrobial and antioxidant coating properties. Comprehensive evaluations on fresh produce demonstrated that the FTN@SNPs wash reduced diverse types of surface pesticide residues by over 86% as quantified by surface-enhanced Raman spectroscopy, outperforming conventional wash solutions. Molecular dynamics simulations reveal that the interactions between pesticide residues and MPNs are primarily formed through π-π interactions, van der Waals forces, and hydrogen bonds. In addition, detailed characterization of the coating's impact on quality parameters, including visual appearance, weight loss, titratable acidity, and total soluble solids, demonstrated its substantial benefits in maintaining postharvest freshness in both whole and fresh-cut produce. This dual-action approach highlights the potential of the FTN@SNPs wash as a sustainable, biodegradable, and scalable strategy to improve food safety and minimize postharvest losses in fresh produce supply chains.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.036
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0010.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.268
Teacher spread0.247 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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