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Record W6884328808 · doi:10.1021/acs.est.2c00406.s001

Triclosan\nis the Predominant Antibacterial Compound\nin Ontario Sewage Sludge

2022· article· en· W6884328808 on OpenAlexaboutno aff

Bibliographic record

VenueFigshare · 2022
Typearticle
Languageen
FieldChemistry
TopicAntimicrobial agents and applications
Canadian institutionsnot available
Fundersnot available
KeywordsTriclosanTriclocarbanSewage sludgeAntibioticsSewageAntibacterial activityEscherichia coli

Abstract

fetched live from OpenAlex

Sewage treatment plants (STPs) accumulate\nboth antibiotic and nonantibiotic\nantimicrobial compounds that can select for antibiotic resistant bacteria.\nHerein, we aimed to identify the predominant antibacterial compounds\nimpacting E. coli from Ontario sewage\nsludge consisting of thousands of unknown compounds. Among the 10\nextracted sludge samples, 6 extracts exerted significant growth inhibition\neffects in E. coli. A total of 103\ncompounds were tentatively detected across the 10 sludge samples by\nsuspect screening, among which the bacterial enoyl-ACP reductase (FabI)\ninhibitor triclocarban was detected at the highest abundance. A hypomorphic\nFabI knockdown E. coli strain was highly\nsusceptible to the sludge extracts, confirming FabI inhibitors as\nthe primary antibacterial compounds in the sludge. Protein affinity\npulldown identified triclosan as the major ligand binding to a His-tagged\nFabI protein from the sludge, despite the higher abundance of triclocarban\nin the same samples. Effect-directed analysis was used to determine\nthe contributions of triclosan to the observed antibacterial potencies.\nAntibacterial effects were only detected in F<sub>17</sub> and F<sub>18</sub> across 20 fractions, which was consistent with the elution\nof triclosan and triclocarban in the same two fractions. Further,\npotency mass balance analysis confirmed that triclosan explained the\nmajority (58–113%) of inhibition effects from sludge extracts.\nThis study highlighted triclosan as the predominant antibacterial\ncompound in sewage sludge impacting E. coli despite the co-occurrence of numerous other antibiotics and nonantibiotics.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.786
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.7870.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.227
Teacher spread0.199 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designNot applicable
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

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