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Record W6921995043 · doi:10.1021/acs.jpca.1c08357.s001

Methods for Interpreting the Partitioning and Fate\nof Petroleum Hydrocarbons in a Sea Ice Environment

2022· article· en· W6921995043 on OpenAlexaboutno aff

Bibliographic record

VenueFigshare · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicOil Spill Detection and Mitigation
Canadian institutionsnot available
Fundersnot available
KeywordsSea iceArcticPetroleumThermokarstAdvectionMesocosmBrineArctic ice pack

Abstract

fetched live from OpenAlex

Decreases\nin Arctic Sea ice extent and thickness have led to more\nopen ice conditions, encouraging both shipping traffic and oil exploration\nwithin the northern Arctic. As a result, the increased potential for\naccidental releases of crude oil or fuel into the Arctic environment\nthreatens the pristine marine environment, its ecosystem, and local\ninhabitants. Thus, there is a need to develop a better understanding\nof oil behavior in a sea ice environment on a microscopic level. Computational\nquantum chemistry was used to simulate the effects of evaporation,\ndissolution, and partitioning within sea ice. Vapor pressures, solubilities,\noctanol–water partition coefficients, and molecular volumes\nwere calculated using quantum chemistry and thermodynamics for pure\nliquid solutes (oil constituents) of interest. These calculations\nincorporated experimentally measured temperatures and salinities taken\nthroughout an oil-in-ice mesocosm experiment conducted at the University\nof Manitoba in 2017. Their potential for interpreting the relative\nmovements of oil constituents was assessed. Our results suggest that\nthe relative movement of oil constituents is influenced by differences\nin physical properties. Lighter molecules showed a greater tendency\nto be controlled by brine advection processes due to their greater\nsolubility. Molecules which are more hydrophobic were found to concentrate\nin areas of lower salt concentration.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.673
Threshold uncertainty score0.960

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0410.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.275
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

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