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Record W6959247633 · doi:10.1021/acs.jpca.0c02679.s004

Climate Metrics for C1–C4 Hydrofluorocarbons\n(HFCs)

2020· article· en· W6959247633 on OpenAlexaboutno aff

Bibliographic record

VenueFigshare · 2020
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicSeed and Plant Biochemistry
Canadian institutionsnot available
Fundersnot available
KeywordsGreenhouse gasGlobal-warming potentialGlobal warmingMetric (unit)Work (physics)Global climateClimate modelRadiative transferRadiative forcing

Abstract

fetched live from OpenAlex

Hydrofluorocarbons\n(HFCs) are potent greenhouse gases that are\npotential substitutes for ozone depleting substances. The Kigali amendment\nlists 17 HFCs that are currently in commercial use to be regulated\nunder the Montreal Protocol. Future commercial applications may explore\nthe use of other HFCs, most of which currently lack an evaluation\nof their climate metrics. In this work, atmospheric lifetimes, radiative\nefficiencies (REs), global warming potentials (GWPs), and global temperature\nchange potentials (GTPs) for all saturated HFCs with fewer than 5\ncarbon atoms are estimated to help guide future usage and policy decisions.\nAtmospheric lifetimes were estimated using a structure activity relationship\n(SAR) for OH radical reactivity and estimated O­(<sup>1</sup>D) reactivity.\nRadiative metrics were obtained using theoretically calculated infrared\nabsorption spectra that were presented in a previous work. Calculations\nfor some additional HFCs not included in the previous work were performed\nin this work. The HFCs display unique infrared spectra with strong\nabsorption in the Earth’s atmospheric infrared window region,\nprimarily due to the C–F stretching vibration. Results from\nthis study show that the HFC global atmospheric lifetimes and REs\nare dependent upon their H atom content and molecular structure. Therefore,\nthe HFC radiative metric evaluation requires a case-by-case evaluation.\nA thorough experimental evaluation of a targeted HFC’s atmospheric\nlifetime and climate metrics is always highly recommended. However,\nin cases where it is experimentally difficult to separate isomers,\nthe new results from this study should help guide the experiments,\nas well as provide relevant climate metrics with uncertainties and\npolicy relevant data.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Dataset · Consensus signal: none
Teacher disagreement score0.711
Threshold uncertainty score0.963

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0380.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.076
GPT teacher head0.219
Teacher spread0.144 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreDataset

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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