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Record W6959671729 · doi:10.11575/prism/dspace/41151

Carbon Dioxide conversion to Carbon nanofibers: Development of the carbonization section

2022· other· en· W6959671729 on OpenAlexaboutno aff

Bibliographic record

VenueUniversity of Calgary · 2022
Typeother
Languageen
Field
Topic
Canadian institutionsnot available
Fundersnot available
KeywordsCarbonizationCarbon nanofiberCarbon fibersExothermic reactionProcess (computing)Carbon dioxideMonolithCarbon dioxide removalHydrogen production

Abstract

fetched live from OpenAlex

Carbon nanofibers (CNFs) have received a great deal of attention as an additive to enhance engineering material properties. In recent years, the use of carbon nanofibers for environmental applications and hydrogen storage has increased due to their high surface area. It is the high cost of CNFs that severely limits their wide application in addition to most of the existing production methods relying on fossil fuels.In the prior art, Dr. M. Zarabian and Dr. Pereira, at the University of Calgary succeeded to develop a net-zero emission technology to produce CNFs from greenhouse gases (GHG) as a feedstock. This M.Sc. thesis aims to evolve the carbonization reactor design to be upscaling-ready by introducing a configuration that could provide uniform reactant concentration, effective transfer of heat generated in exothermic reaction and ease of removing solid fibres. To accomplish this goal, first, the bench-scale method had been fully understood and then new concepts to overcome process bottlenecks were investigated. A new configuration of the reactor to fullfill the requirement was proposed. Then computational fluid dynamics (CFD) was employed to study the flow regime inside the new configuration. Based on CFD results, a prototype of a new configuration was built, and different aspects of process and product were investigated. The results showed that the new reactor configuration to produce carbon nanofiber on sheet metal substrate provides faster nucleation, a more uniform conversion rate and a steady rate of product accumulation compared to monolith configuration. In addition, it shows high up-scalability potential. A prototype of an Autodipping machine was built and successfully employed to impregnate catalysts on the disks. A series of standard characterization procedures for different methods were developed and employed to characterize the products and compare them with commercially available products. The evaluations indicated that both disk and monolith configuration CNF products had comparable and even better features than those of commercial ones.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.477
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.173
Teacher spread0.167 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

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