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Record W6959725226 · doi:10.1021/bc300430k.s001

Rapid Catalyst-Free Hydrazone\nLigation: Protein-Pyridoxal\nPhosphoramides

2016· article· en· W6959725226 on OpenAlexfundno aff

Bibliographic record

VenueFigshare · 2016
Typearticle
Languageen
FieldChemistry
TopicMolecular spectroscopy and chirality
Canadian institutionsnot available
FundersYork University
KeywordsBioorthogonal chemistryPretargetingHydrazideConcanavalin AIn vitro

Abstract

fetched live from OpenAlex

Pyridoxal-5′-phosphate (PLP) represents an active\nform of\nVitamin B<sub>6</sub> that shows relatively fast imine formation with\nhydrazines under physiological conditions without the need of a catalyst.\nA convenient phosphate/amine conjugation protocol was developed to\ncovalently link PLP to proteins, affording proteins capable of hydrazone\nformation with bioorthogonal hydrazinyl functional groups. Thus, the\nlectin Concanavalin A (Con A) was labeled with PLP. Pretreatment with\nfluorescein hydrazide gave dye-labeled Con A that labeled cell surfaces\nefficiently. Alternatively, pretargeting was achieved by labeling\ncells with Con A-PLP, then treatment in vitro with Alexa Fluor 488\nhydrazide.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.792
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.4230.004

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.232
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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