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Record W6989808135

Catalyst-free sequential cure of silicone elastomers by aza-michael addition and thiol-ene photo polymerization

2020· dissertation· en· W6989808135 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueeScholarship@McGill (McGill) · 2020
Typedissertation
Languageen
FieldChemistry
TopicPhotopolymerization techniques and applications
Canadian institutionsnot available
FundersCanadian Institutes of Health ResearchNatural Sciences and Engineering Research Council of CanadaMcGill University
KeywordsElastomerSiliconePolymerizationSilicone ElastomersPolymer
DOInot available

Abstract

fetched live from OpenAlex

FranaisDurant les deux dernires dcennies, d'importants progrs ont t raliss dans le dveloppement de modles in vitro de diffrentes conditions biologiques.Cela a grandement contribu notre comprhension de la faon dont les systmes biologiques interagissent avec leur environnement, comment ils ragissent leurs changements et comment nous pouvons grer cette interaction.Les substrats polymres rigidit accordable ont jou un rle majeur cet gard.Ces polymres peuvent imiter diverses conditions in vivo, du moins du point de vue mcanique, et nous donnent l'occasion de nous rapprocher de ce qui se passe rellement dans notre corps.Cependant, de nombreuses conditions in vivo sont dynamiques et leur mcanique change avec le temps et avec des chelles de temps diffrentes, quelques secondes pour une crise cardiaque et quelques jours pour une tumeur des tissus mous.Cela ncessite la mise au point d'une nouvelle plateforme polymre capable de modifier dynamiquement leur mcanique sur une plage physiologiquement pertinente.Dans ce travail, j'ai dvelopp un nouveau polymre base de silicone partir de ractions par clic aza-Michael et thiol-ne.J'ai montr que les proprits mcaniques de ce nouveau PDMS double durcissement peuvent tre ajustes pour les tapes intermdiaires et finales et j'ai prouv leur structure rseau homogne par analyse thermique.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.062
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.225
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it