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Record W7027240311

Characterization of Multi-Nuclear Manganese-Binding Bacterial Reaction Centers from Rhodobacter sphaeroides

2019· other· en· W7027240311 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueArizona State University Library Digital Repository (Arizona State University) · 2019
Typeother
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicPhotosynthetic Processes and Mechanisms
Canadian institutionsnot available
FundersCanarie
KeywordsRhodobacter sphaeroidesBacteriochlorophyllPhotosynthetic reaction centreManganeseCofactorDimerElectron transferSecondary electrons
DOInot available

Abstract

fetched live from OpenAlex

abstract: In my thesis, I characterize multi-nuclear manganese cofactors in modified reaction \n\ncenters from the bacterium Rhodobacter sphaeroides. I characterized interactions \n\nbetween a variety of secondary electron donors and modified reaction centers. In Chapter \n\n1, I provide the research aims, background, and a summary of the chapters in my thesis. \n\nIn Chapter 2 and Chapter 3, I present my work with artificial four-helix bundles as \n\nsecondary electron donors to modified bacterial reaction centers. In Chapter 2, I \n\ncharacterize the binding and energetics of the P1 Mn-protein, as a secondary electron \n\ndonor to modified reaction centers. In Chapter 3, I present the activity of a suite of four\n\nhelix bundles behaving as secondary electron donors to modified reaction centers. In \n\nChapter 4, I characterize a suite of modified reaction centers designed to bind and oxidize \n\nmanganese. I present work that characterizes bound manganese oxides as secondary \n\nelectron donors to the oxidized bacteriochlorophyll dimer in modified reaction centers. In \n\nChapter 5, I present my conclusions with a short description of future work in \n\ncharacterizing multiple electron transfers from a multi-nuclear manganese cofactor in \n\nmodified reaction centers. To conclude, my thesis presents a characterization of a variety \n\nof secondary electron donors to modified reaction centers that establish the feasibility to \n\ncharacterize multiple turnovers from a multi-nuclear manganese cofactor.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.757
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.153
Teacher spread0.149 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it