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Record W7081965060 · doi:10.1016/j.surfin.2025.107662

Hydrogen peroxide electrochemical sensor using green synthesized silver nanoparticles

2025· article· en· W7081965060 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueSurfaces and Interfaces · 2025
Typearticle
Languageen
FieldComputer Science
TopicGeochemistry and Geologic Mapping
Canadian institutionsMcMaster University
FundersNatural Sciences and Engineering Research Council of CanadaMcMaster Institute for Research on Aging, McMaster UniversityMcMaster University
KeywordsAmperometryAscorbic acidHydrogen peroxideElectrochemical gas sensorSilver nanoparticleGlucose oxidaseDetection limitCyclic voltammetry

Abstract

fetched live from OpenAlex

Green nanomaterial-based electrochemical sensors have attracted considerable attention owing to their biocompatibility, cost-effectiveness, and reduced environmental impact. Hydrogen peroxide (H₂O₂), a key biomarker of oxidative stress associated with aging and various pathologies, requires sensitive and selective detection for reliable biomedical diagnostics. In this work, silver nanoparticles (AgNPs) were synthesized via a green route using orange peel extract (OPE) as both a natural reducing and stabilizing agent, and subsequently employed to fabricate a nonenzymatic H₂O₂ sensor based on AgNP-modified screen-printed carbon electrodes (AgNPs/SPCEs). Structural and spectroscopic characterization confirmed the formation of crystalline AgNPs with an average diameter of ∼32 nm. Electrochemical analysis by cyclic voltammetry demonstrated excellent sensing performance, with dual linear ranges (0.5–10 μM and 10–161.8 μM), a high sensitivity of 20,160 μA mM -1 cm -2 , and a low detection limit of 0.3 μM, S/ N = 3. Amperometric studies demonstrated high selectivity against common interferents such as ascorbic acid, dopamine, glucose, glutamate, and uric acid. The sensor also achieved reliable detection of H₂O₂ in human urine, highlighting its potential for clinical applications. Furthermore, the versatility of the sensing platform was established by immobilizing glucose oxidase onto AgNPs/SPCEs, enabling enzymatic glucose sensing within a physiologically relevant range (3–18 mM). Collectively, these findings establish green-synthesized AgNP-based electrodes as a sustainable, cost-effective, and high-performance platform for the detection of oxidative stress biomarkers and glucose dysregulation in clinical diagnostics.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.044
Threshold uncertainty score0.557

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.236
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it