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Record W7106821169 · doi:10.1016/j.dwt.2025.101588

Comparative performance of functional adsorbent materials for sustainable metal ion recovery

2025· article· en· W7106821169 on OpenAlexaff

Bibliographic record

VenueDesalination and Water Treatment · 2025
Typearticle
Languageen
FieldMaterials Science
TopicMXene and MAX Phase Materials
Canadian institutionsInstitut National de la Recherche Scientifique
FundersH2020 Marie Skłodowska-Curie Actions
KeywordsMXenesAdsorptionMetalMetal ions in aqueous solutionAqueous solutionBET theoryWastewater

Abstract

fetched live from OpenAlex

Heavy metal contamination in water systems poses serious environmental and health risks, necessitating the development of efficient and sustainable treatment technologies. This study explores the adsorption performance of six adsorbent materials for heavy metal removal from aqueous solutions, focusing on two Ti 3 C 2 T x MXenes synthesized through LiF/HCl and NH 4 HF 2 /citric acid etching, commercial activated carbon, α-MnO 2 , and two biomass-derived activated carbons. The materials were characterized using XRD, FTIR, SEM, EDX, and BET analyses, revealing key differences in morphology, surface chemistry, and elemental composition. Adsorption experiments targeting Cr 6+ , Pb 2+ , Zn 2+ , and five other heavy metal ions demonstrated that Ti 3 C 2 T x - NH 4 HF 2 exhibited the highest adsorption capacities due to its delaminated structure and oxygen-rich surface. While other materials like α-MnO 2 and biosourced activated carbons with much higher specific surface area showed moderate to limited performance, the findings reiterate the critical role of surface functionality over plain surface area. The results also highlight how equilibrium-driven experiments at realistic conditions offer a more conservative and reliable assessment compared to previously reported methods. This work supports the potential of functionalized MXenes as promising materials for efficient adsorption of various heavy metal cations in wastewater treatment.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score0.319

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.282
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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