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Record W7113245548

Preferential intergranular oxidation of Alloy X-750 spacers in CANDU off-chemistry environments

2023· article· en· W7113245548 on OpenAlexfundno aff

Bibliographic record

VenueResearch Explorer (The University of Manchester) · 2023
Typearticle
Languageen
FieldMaterials Science
TopicNuclear Materials and Properties
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of CanadaQueen's UniversityUniversity Network of Excellence in Nuclear EngineeringMcMaster University
KeywordsIntergranular corrosionAlloyEmbrittlementStress corrosion crackingInternal oxidationOxidizing agentCarbideCorrosion
DOInot available

Abstract

fetched live from OpenAlex

Preferential intergranular oxidation (PIO) is often suggested as a potential mechanism for primary water stress corrosion cracking (PWSCC) of Alloy 600 (Ni-16Cr-9Fe). Alloy X-750 is a precipitation-hardened variant of Alloy 600 with additional Al and Ti leading to formation of a ϒ’ phase. Alloy X-750 is used for garter spring spacers in CANDU reactor fuel channels, and has experienced irradiation embrittlement in-core. Recognition of the irradiation embrittlement combined with X-750 being a material with known susceptibly to stress corrosion cracking (SCC) in reactor coolant environments, raised questions regarding any plausible risks of SCC to garter springs. While the spacers normally reside in a dry oxidizing mixture of CO2 and O2, extreme, reducing off-chemistry conditions could develop, potentially leading to PIO similar to observations in primary water. Aged and annealed samples of Alloy X-750 were exposed to different CO-CO2 mixtures with the oxygen partial pressure maintained below the NiO dissociation pressure. Internal and intergranular oxidation was observed under these conditions, similar to Alloy 600 exposed to 480 °C hydrogenated steam. Further nanoscale analysis revealed that the presence of intergranular Cr carbides hindered intergranular oxidation. Also, intergranular oxidation of Al and Ti occurred prior to Cr oxidation, suggesting some influence of minor alloying elements in PIO.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.031
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.067
GPT teacher head0.264
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

Explore more

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