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Record W7116342829 · doi:10.5445/ir/1000189070

Quantifying CO emissions from boreal wildfires by assimilating TROPOMI and TCCON observations

2025· article· en· W7116342829 on OpenAlex
Sina Voshtani, Dylan B. A. Jones, Debra Wunch, Drew C. Pendergrass, P. O. Wennberg, David F. Pollard, Isamu Morino, Hirofumi Ohyama, Nicholas M. Deutscher, Frank Hase, Ralf Sussmann, Damien Weidmann, Rigel Kivi, Omaira Torres García, Yao Té, Jack Chen, Kerry Anderson, Robin Stevens, Shobha Kondragunta, Aihua Zhu, Douglas E. J. Worthy, Senen Racki, Kathryn McKain, Maria Makarova, Nicholas Jones, Emmanuel Mahieu, Andrea Cadena-Caicedo, Paolo Cristofanelli, Casper Labuschagne, Elena A. Kozlova, T. Seitz, Martin Steinbacher, Reza Mahdi, Isao Murata

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

aboutThe title or abstract carries a Canadian signal from the geographic lexicon.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueRepository KITopen (Karlsruhe Institute of Technology) · 2025
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsnot available
Fundersnot available
KeywordsData assimilationBorealTroposphereTaigaBiomass burningGreenhouse gasTrace gas

Abstract

fetched live from OpenAlex

We perform a global inverse modelling analysis to quantify biomass burning emissions of carbon monoxide (CO) from the extreme wildfires in Canada between May and September 2023. Using the GEOS-Chem model, we assimilated observations at 3 d temporal and 2° × 2.5° horizontal resolution from the Tropospheric Monitoring Instrument (TROPOMI) separately and then jointly with Total Carbon Column Observing Network (TCCON) measurements. We also evaluated prior emissions from the Quick Fire Emissions Dataset (QFED), Blended Global Biomass Burning Emissions Product eXtended (GBBEPx), Global Fire Assimilation System (GFAS), and Canadian Forest Fire Emissions Prediction System (CFFEPS). The assimilation of TROPOMI-only measurements estimated posterior North America emissions for QFED, GBBEPx, GFAS, and CFFEPS of 110.4 ± 20, 112.8 ± 20, 127.2 ± 17, and 125.6 ± 18 Tg CO compared to prior estimates of 37.1, 42.7, 91.0, and 90.2 Tg CO, respectively. The joint assimilation of TROPOMI+TCCON reduced the posterior 1σ uncertainty on the North American emission estimates by up to about 30 %, while showing only a modest impact (<5 %) on the mean estimate of the inferred emissions. An evaluation against independent measurements reveals that adding TCCON data increases the correlations and slightly lowers the biases and standard deviations. Additionally, including an experimental TCCON product at East Trout Lake with higher surface sensitivity, we find better agreement of the assimilation results with nearby in situ tall tower and aircraft measurements. This highlights the potential importance of vertical sensitivity in these experimental data for constraining local surface emissions. Our results demonstrate the complementarity of the greater temporal coverage provided by TCCON with the spatial coverage of TROPOMI when these data are jointly assimilated.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.297
Threshold uncertainty score0.701

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.255
Teacher spread0.234 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it