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Record W7116661436 · doi:10.1021/acs.jcim.5c02281

Data-Driven Approach for Predicting Gasoline Yield in an FCC Unit Charged with Light and Heavy Feedstocks: A PCA-Guided Grouping for Enhanced Modeling Experience

2025· article· en· W7116661436 on OpenAlexaff
Kawthar Alelg, Azzam Alfarraj, Abdulkadir Tanimu, Saheed A. Ganiyu, K. Alhooshani

Bibliographic record

VenueJournal of Chemical Information and Modeling · 2025
Typearticle
Languageen
FieldEngineering
TopicHeat transfer and supercritical fluids
Canadian institutionsToronto Metropolitan University
FundersKing Fahd University of Petroleum and Minerals
KeywordsCluster analysisLinear regressionRegression analysisKrigingRegressionPartial least squares regressionGasolineData setRobust regressionMixture model

Abstract

fetched live from OpenAlex

This work introduces a feed-aware modeling framework that integrates ensemble anomaly detection, PCA-based segmentation integrated with feed chemistry, and Bayesian-optimized regression to improve the model performance of a Fluid Catalytic Cracking (FCC) unit using pilot-plant experimental data. Three regression models were trained using 5-fold cross-validation and optimized using Bayesian Optimization: Gaussian Process Regression (GPR), Boosted Trees (BT), and Robust Linear Regression (RLR). Modeling on the full unsegmented data set showed that conversion was a highly predictable target. Both GPR and BT achieved strong performance (mean R 2 values of approximately 0.72 to 0.73 after optimization), while RLR remained unstable due to its linear assumptions. For the gasoline yield, BT with optimization performed best (mean R 2 of approximately 0.67), while GPR and RLR with optimization showed limited predictive skill ( R 2 values of approximately 0.25 and −0.51, respectively). These results reflect the nonlinear and distributed nature of yield formation. PCA revealed a clear latent structure that aligned strongly with feedstock type, and K-means clustering confirmed this separation by distinguishing naphtha from VGO samples in a chemically meaningful way. Thus, the data set was segmented into feedstock groups, which yielded substantial improvements, especially for GPR. In the naphtha subset, GPR with optimization achieved mean R 2 values of 0.956 for conversion and 0.902 for gasoline yield, with very low associated error values. Performance also improved for VGO, although to a lesser extent, while RLR continued to underperform. Overall, segmentation based on PCA and clustering was essential for improving model reliability in FCC prediction tasks. Among all algorithms evaluated, GPR consistently delivered the highest accuracy and generalizability across feed types and targets, supporting its suitability for data-driven optimization of catalytic cracking performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.498
Threshold uncertainty score0.444

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.002
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.062
GPT teacher head0.300
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes1
Has abstractyes

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