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Record W7117109761 · doi:10.1016/j.jhazmat.2025.140935

Enhancing separation of oil-in-water slop oil via chemical-assisted centrifugation: Toward scalable and energy-efficient treatment of oil sands waste

2025· article· en· W7117109761 on OpenAlexafffundabout
Yueying Huang, Guangpu Zheng, Ziqian Zhao, Chenyu Qiao, Yimei Sun, Dingzheng Yang, Song Gao, Tian Tang, Hongbo Zeng

Bibliographic record

VenueJournal of Hazardous Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicEnhanced Oil Recovery Techniques
Canadian institutionsNexen (Canada)University of Alberta
FundersCanada's Oil Sands Innovation AllianceNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanada Foundation for Innovation
KeywordsDilutionOil sandsEmulsionTurbidityAsphaltSeparation processCentrifugationProduced waterSolvent

Abstract

fetched live from OpenAlex

Slop oil from oil sands operations presents significant environmental and operational challenges due to its complex composition and stability. This study investigates the separation performance of a field-derived oil-in-water (O/W) slop oil sample from northern Alberta, focusing on centrifugal separation, chemical demulsification, and their integration under the effects of reverse emulsion breaker (REB, branched polyethylenimine), temperature, and dilution. Centrifugal separation was significantly improved by REB addition (optimal dosage: 900 ppm), elevated temperature (70 °C), and organic solvent dilution (e.g., naphtha), enhancing water recovery, reducing turbidity and total organic carbon (TOC) content, and lowering water content in the oil phase. REB exhibited the strongest effect, followed by solvent and thermal treatment, while water dilution hindered separation unless mitigated by REB. Chemical demulsification alone was ineffective. However, when combined with mild centrifugation (5000 rpm, 10 min), REB-assisted treatment achieved results comparable to conventional high-speed centrifugation (7000 rpm, 30 min), while reducing energy input by ∼49 % and cutting process time. Two practical strategies are therefore proposed: (1) solvent dilution followed by high-speed centrifugation for fast bitumen recovery, and (2) REB-assisted mild centrifugation for energy-efficient treatment. This work provides mechanistic insights and practical guidance for the sustainable treatment of oily waste streams in oil sands operations.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.990
Threshold uncertainty score0.020

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.235
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes3
Has abstractyes

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