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Multiphysics modeling and optimization of a methanol-fueled SOFC for distributed power applications

2025· article· en· W7117730484 on OpenAlexafffund
Yannick Poulin-Giroux, Guillaume Jeanmonod, Marie-Lise Tremblay, François Allard

Bibliographic record

VenueJournal of Power Sources · 2025
Typearticle
Languageen
FieldMaterials Science
TopicAdvancements in Solid Oxide Fuel Cells
Canadian institutionsHydro-QuébecUniversité du Québec à Trois-RivièresInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsMultiphysicsSolid oxide fuel cellAnodeElectrical efficiencyElectric potential energyElectric powerCogenerationOverheating (electricity)Chemical energyEnergy transformation

Abstract

fetched live from OpenAlex

A comprehensive multiphysics model of a solid oxide fuel cell (SOFC) system externally fueled by a methanol reforming unit (MRU) is developed and validated using experimental measurements. The model enables a combined analysis of the three main operating concerns: electrical efficiency, energy efficiency, and carbon deposition. A 2D axisymmetric finite element model of the SOFC is coupled with a thermodynamic equilibrium model of the MRU to examine the effects of five operating parameters: temperature, methanol feed rate, steam-to-carbon ratio (S/C), air-to-carbon ratio (A/C), and current density. Both models are validated against experimental data, including GC-MS reformate analysis and polarization curves. A full parametric study is then carried out to assess electrical efficiency and overall energy balance. Results show that temperature is the dominant factor, with nearly a 60 % efficiency drop when decreasing from 850 °C to 750 °C. Increasing S/C slightly improves electrical efficiency but adds a significant thermal penalty, while higher A/C consistently reduces efficiency despite potential heat-balance advantages. The optimal operating window is identified at high temperature (800–850 °C), low methanol feed rate, and low S/C or A/C ratios (0.15–0.3). These conditions maximize electrical efficiency, avoid external energy input, and prevent coke formation at the anode.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.641
Threshold uncertainty score0.359

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.287
Teacher spread0.276 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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