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Record W7132916175

An Investigation on Renewable Carbons as Natural Sources of Fluorescent and Conductive Materials for Smart Device Applications

2023· dissertation· W7132916175 on OpenAlexfundno aff
Maria Natalia Semeniuk

Bibliographic record

VenueTSpace · 2023
Typedissertation
Language
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsnot available
FundersUniversity of Toronto
KeywordsGrapheneCarbon fibersCarbonizationNanoparticlePyrolysisCarbon blackElectrodeCarbon nanotubeHydrothermal carbonization
DOInot available

Abstract

fetched live from OpenAlex

Controlled carbonization of biomass leads to nano-layered graphitic structures with characteristic crystalline sp2 hybridization with conductive and optical properties. The starting material and processing parameters influence the final chemical and morphological structure of the renewable carbon, which determine its practical applications. Biomasses investigated include various wood, xylem sap and peanut shells. Controlled pyrolysis of several wood species to 800 ˚C yielded photoluminescent graphene clusters with a notable electrical conductivity of 600 S/m and electromagnetic interference shielding effectiveness of 47.7 dB at 12 GHz. This is due to the renewable graphitic carbon’s material graphene-graphite composite, since graphene is known to be highly conductive due to its high carrier mobility. Catalytic graphitization with iron nitrate nanoparticles successfully showed the formation of single crystal graphitic carbon structures in black spruce (Picea mariana) at temperatures between 300-800 ˚C and conductivity of 850 S/m. This P. mariana renewable carbon was applied as the cathode of a coin cell battery. To reduce processing temperature further, hydrothermal pyrolysis was performed at 180 ˚C on xylem sap. A characteristic crystalline sp2 carbon was observed in hydrochar xylem syrup. When UV light is shone on the carbon, by the “naked eye” it can selectively detect Fe3+ ions and pH. A chemo sensor was designed based on logic gates, which can displace traditional metal-oxide-semiconductor field-effect transistor (MOSFET) based circuits. Additionally, multiple thermogravimetric comparisons were performed using several model-free and model-based kinetic analyses, where activation energy and pre-exponential factors were determined during the decomposition process. Peanut shell graphitic carbon was applied as an electrode in a Li-ion coin cell battery, yielding a specific capacity of 220 mAh/g and 100 % columbic efficiency for 800 cycles. Thus, these findings on renewable carbon will open a new frontier in sustainable bio-electronics and energy materials manufacturing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.330
Teacher spread0.290 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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