MétaCan
Menu
Back to cohort

Phase separation kinetics

2009· book-chapter· en· W780429120 on OpenAlexaff
Rashmi C. Desai, Raymond Kapral

Bibliographic record

VenueCambridge University Press eBooks · 2009
Typebook-chapter
Languageen
FieldEarth and Planetary Sciences
Topicnanoparticles nucleation surface interactions
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsKineticsStatistical physicsNon-equilibrium thermodynamicsUnderpinningPhase (matter)ThermodynamicsPhysicsEngineeringClassical mechanics

Abstract

fetched live from OpenAlex

Growth of order from disorder is a natural phenomenon which is seen in a variety of systems. An important class of such phenomena involves the kinetics of phase ordering and phase separation. The examples of such growth processes that were described in Chapter 2 had common characteristics. Now, we discuss the experimental results that point to common features of the kinetics of phase separation processes. A combination of techniques from nonequilibrium statistical mechanics and nonlinear dynamics is used to study the formation and evolution of spatial structures. Substantial progress in our understanding of the kinetics of domain growth during a first-order phase transition has been made over the past few decades. The knowledge gained in these studies forms the underpinning of the descriptions of many such processes which create order from disorder. Kinetics of phase ordering and phase separation Phase separation is usually initiated by a rapid change or quench in a thermodynamic variable (often temperature and sometimes pressure), which places a disordered system in a post-quench initial nonequilibrium state. The system then evolves towards an inhomogeneous ordered state of coexisting phases, which is its final equilibrium state. Depending on the nature of the quench, the post-quench state may be either thermodynamically unstable or metastable (see Fig. 2.1). In the former case, the onset of separation is spontaneous, and the kinetics that follows is known as spinodal decomposition. For the metastable case, nonlinear fluctuations are needed to initiate the separation process. The system is said to undergo phase separation through homogeneous nucleation if the system is pure. Phase separation occurs by heterogeneous nucleation if the system has impurities or surfaces which initiate nucleation events.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.025
Threshold uncertainty score0.084

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0020.003
Open science0.0020.001
Research integrity0.0010.003
Insufficient payload (model declined to judge)0.0250.012

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.236
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2009
Admission routes1
Has abstractyes

Explore more

Same venueCambridge University Press eBooksSame topicnanoparticles nucleation surface interactionsFrench-language works237,207