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Record W1640354826 · doi:10.1139/s07-045

High temperature fluidized bed zero valent iron process for flue gas nitrogen monoxide removal

2008· article· en· W1640354826 on OpenAlexvenueno aff
Chih-Yu Cheng, Shiao‐Shing Chen, Chih-Hui Tang, Yu‐Min Chang, Hsu-Hui Cheng, Hsuan‐Liang Liu

Bibliographic record

VenueJournal of Environmental Engineering and Science · 2008
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsnot available
FundersNational Science Council
KeywordsZerovalent ironChemistryFlue gasThermal diffusivityReaction rate constantArrhenius equationEnthalpyActivation energyThermodynamicsCarbon monoxideFluidized bedExothermic reactionNitrogenInorganic chemistryAdsorptionKineticsPhysical chemistryCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

A fluidized bed zero valent iron (ZVI) reactor was designed for nitrogen monoxide (NO) removal with typical flue gas temperatures based on ZVI’s strong reducing abilities. Three different parameters: temperature, influent concentration, and ZVI dosage were tested. Higher NO removals were observed for higher temperature, which was contributed to either higher diffusivity for NO or higher rate constant at higher temperature instead of thermodynamic aspect, since enthalpy change of the chemical reaction (ΔH) is negative and equilibrium constant is decreased when temperature is increased. At the same temperature, ZVI capacities (as mg NO/g ZVI) were constant for both influent concentration and ZVI dosage variation. Activated energies were determined for two different stages: before and after breakthrough. Before breakthrough, excess ZVI was presented and the reaction was described as a pseudo-first order reaction, and the activated energy (Ea) for the first stage was calculated as 46.5 kJ/mol according to the Arrhenius equation. After breakthrough, the presence of ZVI was not in excess and the reaction order of ZVI and NO was considered as 2nd order (1 order in [NO] and 1 order in ZVI), and Ea was determined to be 7.5 kJ/mol.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.209
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2008
Admission routes1
Has abstractyes

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