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Record W1640812498

Raman Spectroscopy Investigations of Tagish Lake Nanodiamonds

2011· article· en· W1640812498 on OpenAlexaboutno aff
T. Jakubowski, Marcin Kozanecki, U. Ott, A. Karczemska

Bibliographic record

VenueMeteoritics and Planetary Science Supplement · 2011
Typearticle
Languageen
FieldMaterials Science
TopicDiamond and Carbon-based Materials Research
Canadian institutionsnot available
Fundersnot available
KeywordsRaman spectroscopyMeteoriteNanodiamondDiamondChondriteAstrobiologyAnalytical Chemistry (journal)Carbonaceous chondriteMaterials scienceChemistryPhysicsOpticsEnvironmental chemistry
DOInot available

Abstract

fetched live from OpenAlex

Introduction: Tagish Lake, a carbonaceous chondrite C2, fell on 18th January 2000 in Canada. According to [1], the meteorite contains about 3650–4330 (ppm) of nanodiamonds, while inferred from measurements of xenon [2] the abundance is 18002500 ppm. This is the highest nanodiamond abundance reported from chondrites. Raman spectroscopic signatures of separated nanodiamonds have been studied in the work presented here. Samples and Experiments: Nanodiamonds were separated following established procedures [3] Raman spectra have been recorded using the confocal Raman micro-spectrometer T-64000 (Jobin-Yvon) with Argon line λ=514.5 nm. Results: The spectra show a diamond peak at 1329 cm (FWHM of about 50 cm) and a broad peak around 1600 cm (Fig.1) [4]. Previous investigations of Allende meteorite presolar nanodiamonds showed peaks at 1326 cm and 1590 cm [5] what is in agreement of laboratory manufactured nanodiamonds Raman investigations [6]. Shifts of diamond peak positions (monocrystalline cubic diamond has Raman peak at 1332 cm) occur because of the nanometer crystal sizes [6] or because of different polytypes [7] of diamond occuring in the sample. References: [1] Grady M. M. et al. (2002) Meteoritics & Planetary Science 37:713-735. [2] Jakubowski T. et al. (2011) Goldschmidt 2011, Abstract #2944. [3] Amari S. et al. (1994) Geochimica et Cosmochimica Acta 58:459-470. [4] Jakubowski T. (2011) PhD thesis, Technical University of Lodz. [5] Gucsik A. et al. (2008) Proceedings of the IAU Symposium 251 “Organic Matter in Space”:335-339. [6] Osswald S. et al. (2009) Physical Review B 80:075419. [7] Phelps A.W. (1999) Lunar and Planetary Science, #1749.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.249
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2011
Admission routes1
Has abstractyes

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