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Record W1880216250 · doi:10.1002/cjce.22135

Experimental and numerical investigation of two‐phase flow patterns in magnesium electrolysis cell with non‐uniform current density distribution

2014· article· en· W1880216250 on OpenAlexvenueno aff
Chenglin Liu, Ze Sun, Guimin Lu, Xingfu Song, Jianguo Yu

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2014
Typearticle
Languageen
FieldEngineering
TopicIndustrial Gas Emission Control
Canadian institutionsnot available
FundersNational Natural Science Foundation of China
KeywordsBubbleMechanicsAnodeCurrent (fluid)Volume fractionMaterials scienceElectrolyteCurrent densityParticle image velocimetryChemistryThermodynamicsAnalytical Chemistry (journal)PhysicsElectrodeTurbulenceChromatography

Abstract

fetched live from OpenAlex

In a magnesium electrolysis cell, the electrolyte flow pattern can be affected by the chlorine gas bubbles release from the anodes. A 2D gas‐liquid mathematical model was developed to simulate the liquid velocity and gas volume fraction. A Particle Image Velocimetry (PIV) experimental set‐up was employed to determine the characteristics of velocity field in a cold model and to validate the mathematical model. The numerical results show good agreement with the experimental data. The local production rate of gas evolution is related to the anode current density according to Faraday's law. To make the bubble generation close to the reality, the non‐uniform current density distribution over the anode surfaces, derived from the thermoelectric model, has been added to the gas‐liquid model as initial boundary conditions. According to the analysis, the use of non‐uniform conditions is necessary. The flow patterns in the side channels are found to be quite different from that in the middle channels, where the velocity is much lower. It is noted that both current intensity and bubble size can significantly affect the velocity field and gas volume fraction distributions. The velocity can be increased with higher current intensities and larger bubble size, and the gas volume fraction can be enhanced with higher current intensities and lower bubble diameters. Additionally, the liquid velocity will decrease sharply when the bubble diameter smaller than the critical value (0.9 mm). It is better to keep the bubble diameter larger than the critical size for the electrolyte circulation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.190
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2014
Admission routes1
Has abstractyes

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