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Record W1909724239 · doi:10.1002/cjce.22318

Iridium‐ruthenium‐oxide coatings for supercapacitors

2015· article· en· W1909724239 on OpenAlexaffvenue
Nehar Ullah, Mark A. McArthur, Sasha Omanovic

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2015
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsMcGill University
Fundersnot available
KeywordsRuthenium oxideMaterials scienceOxideDielectric spectroscopyCyclic voltammetrySupercapacitorElectrochemistryCapacitanceBimetallic stripCoatingChemical engineeringScanning electron microscopeRutheniumElectrodeMetalNanotechnologyMetallurgyComposite materialChemistryCatalysis

Abstract

fetched live from OpenAlex

Abstract Electrochemical, topographical, and morphological properties of thermally‐prepared Irx‐Ru1‐x‐oxide coatings of various compositions (0 < x ≤ 1), formed on a Ti metal substrate, were investigated for their potential application as supercapacitor (SC) electrodes employing scanning electron microscopy and electrochemical techniques of cyclic voltammetry, galvanostatic charge/discharge cycling, and electrochemical impedance spectroscopy. A current state‐of‐the‐art pure ruthenium oxide (RuO2) coating showed relatively low performance compared to other bimetallic IrxRu1‐x‐oxide coatings operated under the same experimental conditions. An electrochemically‐activated Ir0.4Ru0.6‐oxide coating yielded the highest capacitance value (85 mF cm−2). Prolonged electrochemical cycling of the Ir/Ru‐oxide coatings in a corrosive phosphate‐buffered saline pH = 7.4, performed within an extreme potential window of 5 V, revealed an excellent stability of the coatings. In addition, this cycling procedure enabled a significant increase in capacitance for all coating compositions. It was shown that the areal capacitance (CGA) of these coatings is strongly dependent upon the nature of the components of which the metal oxide is composed. The addition of IrO2 to RuO2 improved the stability and capacitive performance of the thermally‐prepared Ir‐Ru‐oxide coatings.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.211
Teacher spread0.187 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2015
Admission routes2
Has abstractyes

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