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Record W1956458658 · doi:10.1139/cjp-2013-0603

Physical and electrical characterization of TiO<sub>2</sub> particles after high temperature processing and before and after ultraviolet irradiation

2014· article· en· W1956458658 on OpenAlexvenueno aff
C. Zúñiga, Mario Moreno, W. Calleja-Arriaga, Pedro Rosales, Roberto Ambrosio, Francisco Javier De la Hidalga, E Gutiérrez, A. Heredia, Erick R. Bandala, José Luis García Sánchez

Bibliographic record

VenueCanadian Journal of Physics · 2014
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsnot available
Fundersnot available
KeywordsRutileIrradiationUltravioletMaterials scienceAnataseAnnealing (glass)Analytical Chemistry (journal)SiliconThin filmBand gapGrain sizeChemical engineeringNanotechnologyPhotocatalysisOptoelectronicsComposite materialPhysicsChemistry

Abstract

fetched live from OpenAlex

In this work, rutile-phase TiO 2 particles (r-TiO 2 , about 360 nm in size) are embedded within a silicon oxide matrix using different concentration ratios of r-TiO 2 with respect to SiO 2 :H 2 O, so that suspensions of mixed TiO 2 :SiO 2 oxides were obtained and analyzed. These TiO 2 :SiO 2 suspensions were deposited on previously-cleaned crystalline silicon and quartz substrates so that thin films of TiO 2 :SiO 2 were obtained. All films were then exposed to relatively high-temperature thermal treatments in nitrogen and different characterization techniques were used to determine their physical and electrical properties before and after ultraviolet (UV) irradiation. Before high thermal treatment, X-ray diffraction patterns show that the main diffraction peaks for the obtained TiO 2 :SiO 2 films correspond to the crystalline phase of rutile-TiO 2 . Infrared analyses before and after thermal treatment show significant changes in the chemical bonding of the final films relative to the temperatures used during annealing. Also, UV–visible spectra provide a constant optical band gap for the films, independent of different TiO 2 concentrations as expected. On the other hand, atomic-force microscopy measurements before and after UV irradiation show an appreciable difference in the grain size and surface morphology of the resulting TiO 2 :SiO 2 oxides annealed at 1000 °C. Finally, photoelectrical I–V properties were obtained for all TiO 2 :SiO 2 films by depositing ultrathin titanium stripes on top of the photoactive material and then, measuring the total current flowing through the metal electrode before and after UV irradiation. From these last measurements, a detectable increase in the I–V slope (lower resistance of the titanium stripe) is found for all samples during UV exposure, thus making this device to act as a simple photoresistor based on r-TiO 2 particles.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.172
Teacher spread0.169 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2014
Admission routes1
Has abstractyes

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